<div>Hi- <br><br>Maybe it is just a naive question. Now I am running the calculation on Lao2 by molpro. As before I used lanl2dz basis set, and it worked fine. But when I change to other basis sets such as ECP28MWB_ANO, it can not run even a rhf calculation. Could you tell me what is happening behind these errors? And is there any special tricks to handle these basis sets?</div>
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<div>Thank you.</div>
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<div>input as</div>
<div>***,laO2 geometry optimization<br> memory,12000,m<br> <br> r=2.21 ang<br> a=67<br> geometry={La;<br> O, La, r<br> O, La, r, O, a}<br> basis=lanl2dz<br>
<br> {rhf<br> occ,7,2,5,1<br> wf,27,1,3}<br> ---<br>runs alright, output RHF-SCF=-180.33591428<br><br>input as <br>***,laO2 geometry optimization <br>memory,12000,m <br><br>r=2.21 ang <br>a=67 <br>
geometry={La; <br>O, La, r <br>O, La, r, O, a} <br>basis= <br>{spdfg,La,ECP28MWB_ANO;c; <br>spdf,o,avtz;c;} <br><br>rhf <br>--- <br>error as <br>Unknown directive RHF-SCF for command MEMORY <br><br>GLOBAL ERROR checkinp on processor 0 <br>
<br>and input <br>***,laO2 geometry optimization <br>memory,12000,m <br><br>r=2.21 ang <br>a=67 <br>geometry={La; <br>O, La, r <br>O, La, r, O, a} <br>basis= <br>{spdfg,La,ECP28MWB_ANO;c; <br>spdf,o,avtz;c;} <br><br>{rhf <br>
occ,13,5,8,3 <br>wf,45,1,3} <br>--- <br>error <br>No subdirectives defined for OCC <br><br>GLOBAL ERROR checkinp on processor 0<br></div>