<div dir="ltr"><div><div>Excuse me, the link for the question on mrcc forum is<br><br><a href="http://www.mrcc.hu/index.php/forum/running-mrcc/81-difference-between-molpro-and-mrcc-fci#376">http://www.mrcc.hu/index.php/forum/running-mrcc/81-difference-between-molpro-and-mrcc-fci#376</a><br><br></div>I am sorry for this inconvenience<br></div><br><div><br></div></div><div class="gmail_extra"><br><div class="gmail_quote">2017-05-25 15:43 GMT-04:00 Cong Wang <span dir="ltr"><<a href="mailto:cwang@chem.helsinki.fi" target="_blank">cwang@chem.helsinki.fi</a>></span>:<br><blockquote class="gmail_quote" style="margin:0 0 0 .8ex;border-left:1px #ccc solid;padding-left:1ex"><div dir="ltr"><div><div><div><div><div><div>Hi everyone,<br><br></div> I tried to compare molpro and mrcc full-ci/cc-pVDZ for a lithium atom and posted my question on mrcc forum.<br><br></div>The molpro convergence pattern is<br><br> 1 1 0.6 1.00000000 -7.43241988<br> <wbr> 0.03 -0.00020840 -0.00020768<br> 2 1 0.6 0.00860636 -7.43263477<br> <wbr> 0.05 -0.00000213 -0.00000210<br> 3 1 0.6 0.00085487 -7.43263690<br> <wbr> 0.09 -0.00000004 -0.00000003<br> 4 1 0.6 0.00009565 -7.43263693<br> <wbr> 0.11 -0.00000000 -0.00000000<br> 5 1 0.6 0.00001648 -7.43263693<br> <wbr> 0.10 -0.00000000 -0.00000000<br> 6 1 0.6 0.00000299 -7.43263693<br> <wbr> 0.12 -0.00000000 -0.00000000<br> 7 1 0.6 0.00000052 -7.43263693<br> <wbr> 0.11 -0.00000000 -0.00000000<br> 8 1 0.6 0.00000010 -7.43263693<br><br></div>mrcc is <br> <br> Iteration 8 CI energy: -7.43263751 Energy decrease: 0.0000E+00<br> =============================<wbr>==============================<wbr>===========<br> Norm of residual vector: 1.0477E-12 Convergence: 5.1862E-12<br> CPU time [min]: 0.012 Wall time [min]: 0.002<br> <br> Iteration 9 CI energy: -7.43263751 Energy decrease: 0.0000E+00<br> =============================<wbr>==============================<wbr>===========<br> Norm of residual vector: 4.7386E-14 Convergence: 2.1137E-13<br> CPU time [min]: 0.013 Wall time [min]: 0.002<br> <br> Iteration 10 CI energy: -7.43263751 Energy decrease: 0.0000E+00<br> =============================<wbr>==============================<wbr>===========<br> Norm of residual vector: 1.8060E-15 Convergence: 1.2633E-14<br> CPU time [min]: 0.014 Wall time [min]: 0.002<br> <br> Iteration 11 CI energy: -7.43263751 Energy decrease: 0.0000E+00<br><br><br></div>Though I was suggested to tighten molpro convergence threshold, my input: <br>{fci;thr,1d-16;core,0}<br></div>and convergence pattern seems unable to reach mrcc value. Hence, I would like to ask in this mailing list, what is the actual reason for this discrepancy? i.e. <br> -7.43263693<br> -7.43263751 <br><br></div>Thank you<br><div><br><div><br></div></div></div>
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