initial guess in molpro

Iwona Dabkowska mega at etoh.chem.univ.gda.pl
Mon Feb 9 12:11:43 GMT 2004


Dear Molpro Support,

Attached, please find two output files, where I want to perform basically
the same calculation -CCSD(T)/6-31G*(0.25) energy of one part of the
system in the basis set of the whole system.
The only difference is that in one case I am asking first for hf en. in
STO-3G basis set, whereas in the other -I am starting from the
default initial guess.
So the result should be the same, but it is not, and in terms of absolute
energy the discrepacy is huge (over 1 Ha).

I am the beginer with Molpro, so maybe I am talking about something well
known, but I find this instability in the wave function very worrying, and
the lack of any warning very misleading.

Also, I would like to know if there is a way to dump the file with guess
during the calculation, so I could start the next one from the given
guess? (not in one job)

Sincerely,
Iwona Dabkowska

****				****
University of Gdansk		Czech Academy of Science
Department of Chemistry    	Center for Complex Molecular Systems and Biomolecules
ul. Sobieskiego 18		Flemingovo n. 2
80-952 Gdansk, POLAND		166 10 Praha 6, CZECH REPUBLIC
phone: +48-58-3450-333		phone: +420-2-20183-333
-------------- next part --------------
ARMCI configured for 4 cluster nodes

 MPP nodes  nproc
 m360         2
 m361         2
 m362         2
 m363         2
 ga_uses_ma=false, calling ma_init with nominal heap. Any -G option will be ignored.

 Primary working directories:    /scratch/mega
 Secondary working directories:  /scratch/mega
 
 blaslib=default         

 MPP tuning parameters: Latency=     5 Microseconds,   Broadcast speed=  300 MB/sec
 default implementation of scratch files=ga  

 Including file /home/scicons/apps/molpro2002.6_intel/bin/molproi.rc
  ***, uu4 planar H-bonded
 ***,uu4 planar H-bonded
  memory,474,M
  
  geometry={option=angstrom,Z;
  O,0,-1.409668,   1.078919,   0.000000;
  C,0,-0.598749,   1.974932,   0.000000;
  N,0, 0.742558,   1.760803,   0.000000;
  C,0, 1.651097,   2.787277,   0.000000;
  C,0, 1.287443,   4.067344,   0.000000;
  C,0,-0.133213,   4.401678,   0.000000;
  N,0,-0.969659,   3.285438,   0.000000;
  O,0,-0.598749,   5.500439,   0.000000;
  H,0, 1.998621,   4.867149,   0.000000;
  H,0, 1.045851,   0.801992,   0.000000;
  H,0,-1.950871,   3.463316,   0.000000;
  H,0, 2.678581,   2.477816,   0.000000;
  O,0, 1.409668,  -1.078919,   0.000000;
  C,0, 0.598749,  -1.974932,   0.000000;
  N,0,-0.742558,  -1.760803,   0.000000;
  C,0,-1.651097,  -2.787277,   0.000000;
  C,0,-1.287443,  -4.067344,   0.000000;
  C,0, 0.133213,  -4.401678,   0.000000;
  N,0, 0.969659,  -3.285438,   0.000000;
  O,0, 0.598749,  -5.500439,   0.000000;
  H,0,-1.998621,  -4.867149,   0.000000;
  H,0,-1.045851,  -0.801992,   0.000000;
  H,0, 1.950871,  -3.463316,   0.000000;
  H,0,-2.678581,  -2.477816,   0.000000}
  
  basis
  sp,n,6-31g;c
  d,n,0.25;
  sp,o,6-31g;c
  d,o,0.25;
  sp,c,6-31g;c
  d,c,0.25;
  sp,h,6-31g;c
  end
  
  
  int;
  DUMMY,1,2,3,4,5,6,7,8,9,10,11,12;
  hf;
  ccsd(t);
  ---

 Variables initialized (303), CPU time= 0.04 sec
 Default parameters read. Elapsed time= 0.06 sec
 Checking input...
 Passed
1


                                         ***  PROGRAM SYSTEM MOLPRO  ***
                                      Copyright, University of Birmingham, 1997

                                    Version 2002.6 linked 15 Dec 2003 19:53:06


 **********************************************************************************************************************************
 LABEL *   UU4 PLANAR H-BONDED                                                           
 Linux-2.4.20-200401280000_bpnnldevelpnnl24_hp4pnnl24smp/m360(ia64) 64 bit mpp version   DATE:   4-Feb-04         TIME: 08:56:29  
 **********************************************************************************************************************************

 Installed patches: configure_xeon dft_orbital_hi enest_dummy fujitsu-ssl2 fujitsu_conf ga_conflict2
                    ia64root_check modelopt molden_orbital_normalization mpputil mxm_fujitsu nec_parse
                    opteron2 patcher_printf posinp readop_multipole_np
 **********************************************************************************************************************************

 Variable memory set to  474000000 words,  buffer space   230000 words
 


 Using spherical harmonics

 Library entry O      S 6-31G                selected for orbital group  1
 Library entry O      P 6-31G                selected for orbital group  1
 Library entry C      S 6-31G                selected for orbital group  2
 Library entry C      P 6-31G                selected for orbital group  2
 Library entry N      S 6-31G                selected for orbital group  3
 Library entry N      P 6-31G                selected for orbital group  3
 Library entry H      S 6-31G                selected for orbital group  4

 Dummy atoms: O  C  N  C  C  C  N  O  H  H  H  H

1PROGRAM * SEWARD (Integral evaluation for generally contracted gaussian basis sets)     Author: Roland Lindh, 1990

 Geometry written to block  1 of record 700


 Point group  Cs  



 ATOMIC COORDINATES

 NR  ATOM    CHARGE       X              Y              Z

   1  O       0.00   -2.663886255    2.038861274    0.000000000
   2  O       0.00   -1.131471546   10.394322527    0.000000000
   3  O       8.00    2.663886255   -2.038861274    0.000000000
   4  O       8.00    1.131471546  -10.394322527    0.000000000
   5  C       0.00   -1.131471546    3.732080326    0.000000000
   6  C       0.00    3.120120911    5.267189784    0.000000000
   7  C       0.00    2.432914496    7.686165661    0.000000000
   8  C       0.00   -0.251736068    8.317965310    0.000000000
   9  C       6.00    1.131471546   -3.732080326    0.000000000
  10  C       6.00   -3.120120911   -5.267189784    0.000000000
  11  C       6.00   -2.432914496   -7.686165661    0.000000000
  12  C       6.00    0.251736068   -8.317965310    0.000000000
  13  N       0.00    1.403231151    3.327435190    0.000000000
  14  N       0.00   -1.832389812    6.208577572    0.000000000
  15  N       7.00   -1.403231151   -3.327435190    0.000000000
  16  N       7.00    1.832389812   -6.208577572    0.000000000
  17  H       0.00    3.776846045    9.197577956    0.000000000
  18  H       0.00    1.976371815    1.515545125    0.000000000
  19  H       0.00   -3.686611629    6.544718252    0.000000000
  20  H       0.00    5.061784128    4.682393290    0.000000000
  21  H       1.00   -3.776846045   -9.197577956    0.000000000
  22  H       1.00   -1.976371815   -1.515545125    0.000000000
  23  H       1.00    3.686611629   -6.544718252    0.000000000
  24  H       1.00   -5.061784128   -4.682393290    0.000000000

 Bond lengths in Bohr (Angstrom)

  1--5  2.283699980   2--8  2.255037428   3--9  2.283699980   4-12  2.255037428   5-13  2.566798677
       (1.208482073)       (1.193314503)       (1.208482073)       (1.193314503)       (1.358291462)

  5-14  2.573776414   6--7  2.514696194   6-13  2.590435935   6-20  2.027817297   7--8  2.757991923
       (1.361983922)       (1.330720014)       (1.370799762)       (1.073074779)       (1.459466579)

  7-17  2.022503185   8-14  2.635902670   9-15  2.566798677   9-16  2.573776414  10-11  2.514696194
       (1.070262671)       (1.394859724)       (1.358291462)       (1.361983922)       (1.330720014)

 10-15  2.590435935  10-24  2.027817297  11-12  2.757991923  11-21  2.022503185  12-16  2.635902670
       (1.370799762)       (1.073074779)       (1.459466579)       (1.070262671)       (1.394859724)

 13-18  1.900377812  14-19  1.884443977  15-22  1.900377812  16-23  1.884443977
       (1.005636703)       (0.997204880)       (1.005636703)       (0.997204880)

 Bond angles

  1--5-13  123.07577386   1--5-14  122.05094466   2--8--7  126.20486319   2--8-14  120.19224842

  3--9-15  123.07577386   3--9-16  122.05094466   4-12-11  126.20486319   4-12-16  120.19224842

  5-13--6  122.44197750   5-13-18  116.62358688   5-14--8  127.35121966   5-14-19  116.07821742

  6--7--8  119.10219759   6--7-17  122.49754050   6-13-18  120.93443562   7--6-13  122.62843538

  7--6-20  122.62073131   7--8-14  113.60288839   8--7-17  118.40026191   8-14-19  116.57056292

  9-15-10  122.44197750   9-15-22  116.62358688   9-16-12  127.35121966   9-16-23  116.07821742

 10-11-12  119.10219759  10-11-21  122.49754050  10-15-22  120.93443562  11-10-15  122.62843538

 11-10-24  122.62073131  11-12-16  113.60288839  12-11-21  118.40026191  12-16-23  116.57056292

 13--5-14  114.87328149  13--6-20  114.75083331  15--9-16  114.87328149  15-10-24  114.75083331

 NUCLEAR CHARGE:                   58
 NUMBER OF PRIMITIVE AOS:         480
 NUMBER OF SYMMETRY AOS:          464
 NUMBER OF CONTRACTIONS:          240   ( 176A'  +  64A"  )
 NUMBER OF CORE ORBITALS:           8   (   8A'  +   0A"  )
 NUMBER OF VALENCE ORBITALS:       36   (  28A'  +   8A"  )


 NUCLEAR REPULSION ENERGY  360.46121681


 Eigenvalues of metric

         1 0.112E-03 0.113E-03 0.407E-03 0.422E-03 0.505E-03 0.546E-03 0.792E-03 0.798E-03
         2 0.112E-01 0.118E-01 0.196E-01 0.208E-01 0.285E-01 0.294E-01 0.302E-01 0.306E-01
 

 Contracted 2-electron integrals neglected if value below      1.0D-11
 AO integral compression algorithm  1   Integral accuracy      1.0D-11

     419.955 MB (compressed) written to integral file ( 29.2%)

     Node minimum: 50.594 MB, node maximum: 55.050 MB
 

 NUMBER OF SORTED TWO-ELECTRON INTEGRALS:   27591744.     BUFFER LENGTH:  32768
 NUMBER OF SEGMENTS:   2  SEGMENT LENGTH:   15956472      RECORD LENGTH: 524288

 Memory used in sort:      16.51 MW

 SORT1 READ  179622569. AND WROTE   13095750. INTEGRALS IN   39 RECORDS. CPU TIME:    15.92 SEC, REAL TIME:    16.30 SEC
 SORT2 READ  105057693. AND WROTE  220672156. INTEGRALS IN 1680 RECORDS. CPU TIME:     1.88 SEC, REAL TIME:     2.81 SEC

 Node minimum:   27576295.  Node maximum:   27591744. integrals

 OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000    0.000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        4.44       600      500      700      960      900      950      970     1000     1100     1400   
                                        BASINP     VAR     GEOM    ABASIS   SYMINP    ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
 PROGRAMS   *        TOTAL       INT
 CPU TIMES  *        31.02     30.84
 REAL TIME  *        33.08 SEC
 DISK USED  *         1.70 GB
 GA USED    *         0.00 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************

1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner


 NUMBER OF ELECTRONS:      29+   29-
 CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
 MAX. NUMBER OF ITERATIONS:       60
 INTERPOLATION TYPE:            DIIS
 INTERPOLATION STEPS:              2 (START)      1 (STEP)
 LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN) 



 
 Molecular orbital dump at record        2100.2

 ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.            DIPOLE MOMENTS         DIIS
    1      0.000D+00      0.000D+00      -356.02295605   1271.955567 -16.554643 -17.223834   0.000000    0
    2      0.000D+00      0.440D-01      -378.88050640   1119.996538  14.473711  19.982193   0.000000    0
    3      0.303D+00      0.618D-01      -335.63403658   1196.406291 -40.980481 -61.302547   0.000000    1
    4      0.435D+00      0.895D-01      -401.05263512   1039.264939   1.878831  30.115061   0.000000    2
    5      0.440D+00      0.433D-01      -393.65495884   1001.974941   4.318637 -57.173772   0.000000    3
    6      0.246D+00      0.498D-01      -410.12620168   1008.815328  -8.151861  10.504959   0.000000    4
    7      0.261D+00      0.151D-01      -410.36562456    992.964985  10.901302  -4.198260   0.000000    5
    8      0.190D+00      0.147D-01      -411.53325196    988.144413  -0.531406  -9.719307   0.000000    6
    9      0.612D-01      0.363D-02      -411.61932767    995.806181   0.689309  -5.193459   0.000000    7
   10      0.347D-01      0.933D-03      -411.62872525    995.900933   0.322749  -5.005167   0.000000    8
   11      0.104D-01      0.584D-03      -411.63240855    996.117741   0.423602  -4.629323   0.000000    9
   12      0.639D-02      0.351D-03      -411.63428789    996.512952   0.433511  -4.374386   0.000000    9
   13      0.554D-02      0.241D-03      -411.63511698    996.734065   0.497257  -4.100517   0.000000    9
   14      0.379D-02      0.148D-03      -411.63537670    996.812303   0.500633  -4.042482   0.000000    9
   15      0.127D-02      0.727D-04      -411.63553252    996.895818   0.524713  -3.932384   0.000000    9
   16      0.152D-02      0.442D-04      -411.63559827    996.928987   0.522491  -3.914366   0.000000    9
   17      0.959D-03      0.308D-04      -411.63565523    996.965170   0.541284  -3.849334   0.000000    9
   18      0.139D-02      0.182D-04      -411.63567328    996.985351   0.546512  -3.829878   0.000000    9
   19      0.975D-03      0.109D-04      -411.63568039    997.002726   0.557659  -3.802929   0.000000    9
   20      0.798D-03      0.502D-05      -411.63568111    997.000996   0.559790  -3.800020   0.000000    9
   21      0.251D-03      0.165D-05      -411.63568122    997.001457   0.561092  -3.797909   0.000000    9
   22      0.884D-04      0.765D-06      -411.63568124    997.000616   0.561204  -3.798324   0.000000    9
   23      0.296D-04      0.377D-06      -411.63568124    997.000358   0.561527  -3.797695   0.000000    9
   24      0.280D-04      0.260D-06      -411.63568125    996.999917   0.561465  -3.798034   0.000000    9
   25      0.912D-05      0.141D-06      -411.63568125    996.999987   0.561536  -3.797863   0.000000    0
 
 Final occupancy:  25   4

 !RHF STATE 1.1 ENERGY               -411.63568125
 Nuclear energy                       360.46121681
 One-electron energy                -1270.59689179
 Two-electron energy                  498.49999373
 Virial quotient                       -0.99745750
 !RHF STATE 1.1 DIPOLE MOMENTS:         0.56153589    -3.79786311     0.00000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        4.49       600      500      700      960      900      950      970     1000     1100     1400   
                                        BASINP     VAR     GEOM    ABASIS   SYMINP    ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
              2       3        1.17       700     1000     2100   
                                         GEOM     BASIS     RHF  
 
 PROGRAMS   *        TOTAL    HF-SCF       INT
 CPU TIMES  *        51.90     20.88     30.84
 REAL TIME  *        54.52 SEC
 DISK USED  *         1.80 GB
 GA USED    *         0.14 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************


1PROGRAM * CCSD (Closed-shell coupled cluster)     Authors: C. Hampel, H.-J. Werner, 1991, M. Deegan, P.J. Knowles, 1992


 Convergence thresholds:  THRVAR = 1.00D-10  THRDEN = 1.00D-06

 CCSD(T)     terms to be evaluated (factor= 1.000)


 Number of core orbitals:           8 (   8   0 )
 Number of closed-shell orbitals:  21 (  17   4 )
 Number of external orbitals:     211 ( 151  60 )

 Setting scratch file implementation to df  

 
 Molecular orbitals read from record     2100.2  Type=RHF/CANONICAL (state 1.1)

 Number of N-1 electron functions:              21
 Number of N-2 electron functions:             231
 Number of singly external CSFs:              2807
 Number of doubly external CSFs:           5260528
 Total number of CSFs:                     5263336

 Length of J-op  integral file:      0.00 MB
 Length of K-op  integral file:      2.19 MB
 Length of 3-ext integral record:    0.00 MB

 Integral transformation finished. Total CPU:  47.10 sec, npass=  1  Memory used:  57.81 MW

 Reference energy:                   -411.63568125
 MP2 correlation energy:               -1.03201834
 MP2 total energy:                   -412.66769958

 ITER.       NORM       CORR.ENERGY   TOTAL ENERGY   ENERGY CHANGE        DEN1      VAR(S)    VAR(P)  DIIS     TIME
   1      1.43320039    -0.97198644  -412.60766769     0.06003190    -0.06319896  0.28D-01  0.23D-01  0  0    86.65
   2      1.49578452    -1.01601593  -412.65169718    -0.04402949    -0.00769666  0.90D-03  0.84D-02  0  0   126.15
   3      1.53232769    -1.01687956  -412.65256081    -0.00086363    -0.00216291  0.21D-02  0.12D-01  1  1   165.79
   4      1.58549703    -1.01944678  -412.65512803    -0.00256722    -0.00380898  0.98D-03  0.30D-01  2  2   206.14
   5      1.53910400    -1.01878761  -412.65446885     0.00065918    -0.00183826  0.10D-02  0.12D-01  3  3   246.34
   6      1.53658091    -1.02244222  -412.65812347    -0.00365461    -0.00073175  0.31D-03  0.10D-02  4  4   286.75
   7      1.57391152    -1.02609118  -412.66177242    -0.00364896    -0.00044489  0.17D-03  0.16D-02  5  5   327.03
   8      1.56934924    -1.02615240  -412.66183365    -0.00006123    -0.00039042  0.19D-03  0.12D-02  6  6   367.43
   9      1.56378547    -1.02631471  -412.66199596    -0.00016231    -0.00019920  0.15D-03  0.36D-03  6  4   407.95
  10      1.58398763    -1.02709791  -412.66277916    -0.00078320    -0.00012285  0.53D-04  0.25D-03  6  3   448.60
  11      1.59306647    -1.02724717  -412.66292841    -0.00014925    -0.00012776  0.38D-04  0.32D-03  6  2   489.23
  12      1.59148592    -1.02738247  -412.66306372    -0.00013531    -0.00011933  0.39D-04  0.30D-03  6  1   529.92
  13      1.58953397    -1.02734053  -412.66302178     0.00004194    -0.00012040  0.43D-04  0.29D-03  6  5   570.55
  14      1.59026665    -1.02739718  -412.66307843    -0.00005665    -0.00011619  0.41D-04  0.26D-03  6  3   611.27
  15      1.59315174    -1.02742444  -412.66310569    -0.00002726    -0.00012271  0.34D-04  0.31D-03  6  3   652.15
  16      1.58938603    -1.02740203  -412.66308327     0.00002241    -0.00011268  0.42D-04  0.26D-03  6  3   692.88
  17      1.59295105    -1.02744626  -412.66312751    -0.00004424    -0.00012003  0.32D-04  0.35D-03  6  3   733.75
  18      1.58394084    -1.02738336  -412.66306461     0.00006290    -0.00010346  0.45D-04  0.21D-03  6  6   774.30
  19      1.58298445    -1.02759909  -412.66328034    -0.00021573    -0.00008348  0.42D-04  0.17D-03  6  4   814.70
  20      1.58365007    -1.02760660  -412.66328784    -0.00000750    -0.00008641  0.36D-04  0.22D-03  6  1   855.38
  21      1.58364315    -1.02765107  -412.66333232    -0.00004448    -0.00007086  0.34D-04  0.16D-03  6  5   895.67
  22      1.58796697    -1.02770792  -412.66338917    -0.00005685    -0.00004708  0.28D-04  0.91D-04  6  3   936.00
  23      1.59066528    -1.02761719  -412.66329843     0.00009073    -0.00003591  0.20D-04  0.13D-03  6  4   976.37
  24      1.59876648    -1.02757582  -412.66325707     0.00004137    -0.00002936  0.75D-05  0.11D-03  6  6  1016.65
  25      1.59881816    -1.02765530  -412.66333654    -0.00007948    -0.00003616  0.84D-05  0.20D-03  6  2  1056.89
  26      1.60070936    -1.02757223  -412.66325348     0.00008306    -0.00002468  0.52D-05  0.63D-04  6  6  1097.10
  27      1.60840494    -1.02786015  -412.66354139    -0.00028792    -0.00002096  0.32D-05  0.53D-04  6  3  1137.68
  28      1.61185938    -1.02785168  -412.66353292     0.00000847    -0.00002032  0.14D-05  0.51D-04  6  4  1178.13
  29      1.61255491    -1.02785490  -412.66353615    -0.00000322    -0.00002074  0.13D-05  0.55D-04  6  1  1218.65

 Norm of t1 vector:      0.08898934      S-energy:     0.00000042      T1 diagnostic:  0.03254838
 Norm of t2 vector:      0.52356557      P-energy:    -1.02785532

 ?CONVERGENCE NOT REACHED AFTER MAX. ITERATIONS

 Memory could be reduced to 132.8 Mword without degradation in triples

 CPU time for triples:    739.28 sec


 RESULTS
 =======
 !CCSD ENERGY                        -412.663536146874
 !CCSD[T] ENERGY                     -412.739301317449     (Triples contribution  -0.07576517)
 !CCSD-T ENERGY                      -412.728956931610     (Triples contribution  -0.06542078)

 Reference energy                    -411.635681246634
 Correlation energy                    -1.095445715959
 !CCSD(T) ENERGY                     -412.731126962594     (Triples contribution  -0.06759082)

 Program statistics:

 Available memory in ccsd:               473999018
 Min. memory needed in ccsd:              12823789
 Max. memory used in ccsd:                17690791
 Max. memory used in cckext:              16918186 (29 integral passes)



 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      19      511.27       600      500      700      960      900      950      970     1000     1100     1400   
                                        BASINP     VAR     GEOM    ABASIS   SYMINP    ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700     1380   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER     JKOP   
 
              2       3        1.17       700     1000     2100   
                                         GEOM     BASIS     RHF  
 
 PROGRAMS   *        TOTAL   CCSD(T)    HF-SCF       INT
 CPU TIMES  *      2009.87   1957.96     20.88     30.84
 REAL TIME  *      2166.50 SEC
 DISK USED  *        12.87 GB
 GA USED    *         0.14 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************

        CCSD(T)         HF-SCF  
   -412.73112696   -411.63568125
 **********************************************************************************************************************************
 Variable memory released
-------------- next part --------------
ARMCI configured for 4 cluster nodes

 MPP nodes  nproc
 m80          2
 m81          2
 m82          2
 m83          2
 ga_uses_ma=false, calling ma_init with nominal heap. Any -G option will be ignored.

 Primary working directories:    /scratch/mega
 Secondary working directories:  /scratch/mega
 
 blaslib=default         

 MPP tuning parameters: Latency=     5 Microseconds,   Broadcast speed=  300 MB/sec
 default implementation of scratch files=ga  

 Including file /home/scicons/apps/molpro2002.6_intel/bin/molproi.rc
  ***, uu4 planar H-bonded
 ***,uu4 planar H-bonded
  memory,475,M
  
  geometry={option=angstrom,Z;
  O,0,-1.409668,   1.078919,   0.000000;
  C,0,-0.598749,   1.974932,   0.000000;
  N,0, 0.742558,   1.760803,   0.000000;
  C,0, 1.651097,   2.787277,   0.000000;
  C,0, 1.287443,   4.067344,   0.000000;
  C,0,-0.133213,   4.401678,   0.000000;
  N,0,-0.969659,   3.285438,   0.000000;
  O,0,-0.598749,   5.500439,   0.000000;
  H,0, 1.998621,   4.867149,   0.000000;
  H,0, 1.045851,   0.801992,   0.000000;
  H,0,-1.950871,   3.463316,   0.000000;
  H,0, 2.678581,   2.477816,   0.000000;
  O,0, 1.409668,  -1.078919,   0.000000;
  C,0, 0.598749,  -1.974932,   0.000000;
  N,0,-0.742558,  -1.760803,   0.000000;
  C,0,-1.651097,  -2.787277,   0.000000;
  C,0,-1.287443,  -4.067344,   0.000000;
  C,0, 0.133213,  -4.401678,   0.000000;
  N,0, 0.969659,  -3.285438,   0.000000;
  O,0, 0.598749,  -5.500439,   0.000000;
  H,0,-1.998621,  -4.867149,   0.000000;
  H,0,-1.045851,  -0.801992,   0.000000;
  H,0, 1.950871,  -3.463316,   0.000000;
  H,0,-2.678581,  -2.477816,   0.000000}
  
  basis=STO-3G;
  DUMMY,1,2,3,4,5,6,7,8,9,10,11,12;
  hf;
  
  basis
  sp,n,6-31g;c
  d,n,0.25;
  sp,o,6-31g;c
  d,o,0.25;
  sp,c,6-31g;c
  d,c,0.25;
  sp,h,6-31g;c
  end
  
  
  int;
  DUMMY,1,2,3,4,5,6,7,8,9,10,11,12;
  hf;
  ccsd(t);
  ---

 Variables initialized (303), CPU time= 0.04 sec
 Default parameters read. Elapsed time= 0.06 sec
 Checking input...
 Passed
1


                                         ***  PROGRAM SYSTEM MOLPRO  ***
                                      Copyright, University of Birmingham, 1997

                                    Version 2002.6 linked 15 Dec 2003 19:53:06


 **********************************************************************************************************************************
 LABEL *   UU4 PLANAR H-BONDED                                                           
 Linux-2.4.20-200401280000_bpnnldevelpnnl24_hp4pnnl24smp/m80(ia64) 64 bit mpp version    DATE:   5-Feb-04         TIME: 05:45:43  
 **********************************************************************************************************************************

 Installed patches: configure_xeon dft_orbital_hi enest_dummy fujitsu-ssl2 fujitsu_conf ga_conflict2
                    ia64root_check modelopt molden_orbital_normalization mpputil mxm_fujitsu nec_parse
                    opteron2 patcher_printf posinp readop_multipole_np
 **********************************************************************************************************************************
 SETTING BASIS          =    STO-3G

 Variable memory set to  475000000 words,  buffer space   230000 words
 

 Dummy atoms: O  C  N  C  C  C  N  O  H  H  H  H


 Using spherical harmonics

 Library entry O      S STO-3G               selected for orbital group  1
 Library entry O      P STO-3G               selected for orbital group  1
 Library entry C      S STO-3G               selected for orbital group  2
 Library entry C      P STO-3G               selected for orbital group  2
 Library entry N      S STO-3G               selected for orbital group  3
 Library entry N      P STO-3G               selected for orbital group  3
 Library entry H      S STO-3G               selected for orbital group  4

1PROGRAM * SEWARD (Integral evaluation for generally contracted gaussian basis sets)     Author: Roland Lindh, 1990

 Geometry written to block  1 of record 700


 Point group  Cs  



 ATOMIC COORDINATES

 NR  ATOM    CHARGE       X              Y              Z

   1  O       0.00   -2.663886255    2.038861274    0.000000000
   2  O       0.00   -1.131471546   10.394322527    0.000000000
   3  O       8.00    2.663886255   -2.038861274    0.000000000
   4  O       8.00    1.131471546  -10.394322527    0.000000000
   5  C       0.00   -1.131471546    3.732080326    0.000000000
   6  C       0.00    3.120120911    5.267189784    0.000000000
   7  C       0.00    2.432914496    7.686165661    0.000000000
   8  C       0.00   -0.251736068    8.317965310    0.000000000
   9  C       6.00    1.131471546   -3.732080326    0.000000000
  10  C       6.00   -3.120120911   -5.267189784    0.000000000
  11  C       6.00   -2.432914496   -7.686165661    0.000000000
  12  C       6.00    0.251736068   -8.317965310    0.000000000
  13  N       0.00    1.403231151    3.327435190    0.000000000
  14  N       0.00   -1.832389812    6.208577572    0.000000000
  15  N       7.00   -1.403231151   -3.327435190    0.000000000
  16  N       7.00    1.832389812   -6.208577572    0.000000000
  17  H       0.00    3.776846045    9.197577956    0.000000000
  18  H       0.00    1.976371815    1.515545125    0.000000000
  19  H       0.00   -3.686611629    6.544718252    0.000000000
  20  H       0.00    5.061784128    4.682393290    0.000000000
  21  H       1.00   -3.776846045   -9.197577956    0.000000000
  22  H       1.00   -1.976371815   -1.515545125    0.000000000
  23  H       1.00    3.686611629   -6.544718252    0.000000000
  24  H       1.00   -5.061784128   -4.682393290    0.000000000

 Bond lengths in Bohr (Angstrom)

  1--5  2.283699980   2--8  2.255037428   3--9  2.283699980   4-12  2.255037428   5-13  2.566798677
       (1.208482073)       (1.193314503)       (1.208482073)       (1.193314503)       (1.358291462)

  5-14  2.573776414   6--7  2.514696194   6-13  2.590435935   6-20  2.027817297   7--8  2.757991923
       (1.361983922)       (1.330720014)       (1.370799762)       (1.073074779)       (1.459466579)

  7-17  2.022503185   8-14  2.635902670   9-15  2.566798677   9-16  2.573776414  10-11  2.514696194
       (1.070262671)       (1.394859724)       (1.358291462)       (1.361983922)       (1.330720014)

 10-15  2.590435935  10-24  2.027817297  11-12  2.757991923  11-21  2.022503185  12-16  2.635902670
       (1.370799762)       (1.073074779)       (1.459466579)       (1.070262671)       (1.394859724)

 13-18  1.900377812  14-19  1.884443977  15-22  1.900377812  16-23  1.884443977
       (1.005636703)       (0.997204880)       (1.005636703)       (0.997204880)

 Bond angles

  1--5-13  123.07577386   1--5-14  122.05094466   2--8--7  126.20486319   2--8-14  120.19224842

  3--9-15  123.07577386   3--9-16  122.05094466   4-12-11  126.20486319   4-12-16  120.19224842

  5-13--6  122.44197750   5-13-18  116.62358688   5-14--8  127.35121966   5-14-19  116.07821742

  6--7--8  119.10219759   6--7-17  122.49754050   6-13-18  120.93443562   7--6-13  122.62843538

  7--6-20  122.62073131   7--8-14  113.60288839   8--7-17  118.40026191   8-14-19  116.57056292

  9-15-10  122.44197750   9-15-22  116.62358688   9-16-12  127.35121966   9-16-23  116.07821742

 10-11-12  119.10219759  10-11-21  122.49754050  10-15-22  120.93443562  11-10-15  122.62843538

 11-10-24  122.62073131  11-12-16  113.60288839  12-11-21  118.40026191  12-16-23  116.57056292

 13--5-14  114.87328149  13--6-20  114.75083331  15--9-16  114.87328149  15-10-24  114.75083331

 NUCLEAR CHARGE:                   58
 NUMBER OF PRIMITIVE AOS:         264
 NUMBER OF SYMMETRY AOS:          264
 NUMBER OF CONTRACTIONS:           88   (  72A'  +  16A"  )
 NUMBER OF CORE ORBITALS:           8   (   8A'  +   0A"  )
 NUMBER OF VALENCE ORBITALS:       36   (  28A'  +   8A"  )


 NUCLEAR REPULSION ENERGY  360.46121681


 Eigenvalues of metric

         1 0.180E+00 0.180E+00 0.217E+00 0.218E+00 0.219E+00 0.219E+00 0.244E+00 0.245E+00
         2 0.604E+00 0.605E+00 0.703E+00 0.704E+00 0.751E+00 0.751E+00 0.976E+00 0.978E+00
 

 Contracted 2-electron integrals neglected if value below      1.0D-11
 AO integral compression algorithm  1   Integral accuracy      1.0D-11

     12.583 MB (compressed) written to integral file ( 55.9%)

     Node minimum: 1.573 MB, node maximum: 1.573 MB
 

 NUMBER OF SORTED TWO-ELECTRON INTEGRALS:     566900.     BUFFER LENGTH:  32768
 NUMBER OF SEGMENTS:   1  SEGMENT LENGTH:     566900      RECORD LENGTH: 524288

 Memory used in sort:       1.12 MW

 SORT1 READ    2850304. AND WROTE     235733. INTEGRALS IN    1 RECORDS. CPU TIME:     0.60 SEC, REAL TIME:     0.62 SEC
 SORT2 READ    1895029. AND WROTE    4536046. INTEGRALS IN   48 RECORDS. CPU TIME:     0.03 SEC, REAL TIME:     0.05 SEC

 Node minimum:     565865.  Node maximum:     568148. integrals

 OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000    0.000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        3.36       600      500      700      960      900      950      970     1000     1100     1400   
                                        BASINP     VAR     GEOM    ABASIS   SYMINP    ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
 PROGRAMS   *        TOTAL       INT
 CPU TIMES  *         2.28      2.04
 REAL TIME  *         2.60 SEC
 DISK USED  *        41.28 MB
 GA USED    *         0.00 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************
1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner


 NUMBER OF ELECTRONS:      29+   29-
 CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
 MAX. NUMBER OF ITERATIONS:       60
 INTERPOLATION TYPE:            DIIS
 INTERPOLATION STEPS:              2 (START)      1 (STEP)
 LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN) 



 
 Orbital guess generated from atomic densities.  Occupancy:   25   5
 Molecular orbital dump at record        2100.2

 ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.            DIPOLE MOMENTS         DIIS
    1      0.000D+00      0.000D+00      -406.76472714   1009.162006  -2.577136   1.567939   0.000000    0
    2      0.000D+00      0.182D-01      -406.90059252   1016.319699  -0.084236   0.086781   0.000000    1
    3      0.363D-01      0.158D-01      -407.07190825   1012.289421  -1.197892   0.525950   0.000000    2
    4      0.157D-01      0.127D-02      -407.07551761   1012.375837  -1.168437   0.532021   0.000000    3
    5      0.263D-02      0.579D-03      -407.07615482   1012.309303  -1.154009   0.489767   0.000000    4
    6      0.121D-02      0.214D-03      -407.07624774   1012.293621  -1.153308   0.493416   0.000000    5
    7      0.528D-03      0.714D-04      -407.07625496   1012.291317  -1.151908   0.490971   0.000000    6
    8      0.132D-03      0.299D-04      -407.07625637   1012.287505  -1.151563   0.490112   0.000000    7
    9      0.697D-04      0.678D-05      -407.07625644   1012.286859  -1.151428   0.490160   0.000000    8
   10      0.149D-04      0.200D-05      -407.07625644   1012.286712  -1.151455   0.489918   0.000000    7
   11      0.369D-05      0.503D-06      -407.07625644   1012.286840  -1.151404   0.489948   0.000000    0
 
 Final occupancy:  24   5

 !RHF STATE 1.1 ENERGY               -407.07625644
 Nuclear energy                       360.46121681
 One-electron energy                -1273.68089333
 Two-electron energy                  506.14342007
 Virial quotient                       -1.00876889
 !RHF STATE 1.1 DIPOLE MOMENTS:        -1.15140412     0.48994794     0.00000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        3.37       600      500      700      960      900      950      970     1000     1100     1400   
                                        BASINP     VAR     GEOM    ABASIS   SYMINP    ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
              2       3        0.55       700     1000     2100   
                                         GEOM     BASIS     RHF  
 
 PROGRAMS   *        TOTAL    HF-SCF       INT
 CPU TIMES  *         2.54      0.27      2.04
 REAL TIME  *         2.87 SEC
 DISK USED  *        80.31 MB
 GA USED    *         0.02 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************


 Using spherical harmonics

 Library entry O      S 6-31G                selected for orbital group  1
 Library entry O      P 6-31G                selected for orbital group  1
 Library entry C      S 6-31G                selected for orbital group  2
 Library entry C      P 6-31G                selected for orbital group  2
 Library entry N      S 6-31G                selected for orbital group  3
 Library entry N      P 6-31G                selected for orbital group  3
 Library entry H      S 6-31G                selected for orbital group  4

 Dummy atoms: O  C  N  C  C  C  N  O  H  H  H  H

1PROGRAM * SEWARD (Integral evaluation for generally contracted gaussian basis sets)     Author: Roland Lindh, 1990

 Geometry written to block  1 of record 700


 Point group  Cs  



 ATOMIC COORDINATES

 NR  ATOM    CHARGE       X              Y              Z

   1  O       0.00   -2.663886255    2.038861274    0.000000000
   2  O       0.00   -1.131471546   10.394322527    0.000000000
   3  O       8.00    2.663886255   -2.038861274    0.000000000
   4  O       8.00    1.131471546  -10.394322527    0.000000000
   5  C       0.00   -1.131471546    3.732080326    0.000000000
   6  C       0.00    3.120120911    5.267189784    0.000000000
   7  C       0.00    2.432914496    7.686165661    0.000000000
   8  C       0.00   -0.251736068    8.317965310    0.000000000
   9  C       6.00    1.131471546   -3.732080326    0.000000000
  10  C       6.00   -3.120120911   -5.267189784    0.000000000
  11  C       6.00   -2.432914496   -7.686165661    0.000000000
  12  C       6.00    0.251736068   -8.317965310    0.000000000
  13  N       0.00    1.403231151    3.327435190    0.000000000
  14  N       0.00   -1.832389812    6.208577572    0.000000000
  15  N       7.00   -1.403231151   -3.327435190    0.000000000
  16  N       7.00    1.832389812   -6.208577572    0.000000000
  17  H       0.00    3.776846045    9.197577956    0.000000000
  18  H       0.00    1.976371815    1.515545125    0.000000000
  19  H       0.00   -3.686611629    6.544718252    0.000000000
  20  H       0.00    5.061784128    4.682393290    0.000000000
  21  H       1.00   -3.776846045   -9.197577956    0.000000000
  22  H       1.00   -1.976371815   -1.515545125    0.000000000
  23  H       1.00    3.686611629   -6.544718252    0.000000000
  24  H       1.00   -5.061784128   -4.682393290    0.000000000

 Bond lengths in Bohr (Angstrom)

  1--5  2.283699980   2--8  2.255037428   3--9  2.283699980   4-12  2.255037428   5-13  2.566798677
       (1.208482073)       (1.193314503)       (1.208482073)       (1.193314503)       (1.358291462)

  5-14  2.573776414   6--7  2.514696194   6-13  2.590435935   6-20  2.027817297   7--8  2.757991923
       (1.361983922)       (1.330720014)       (1.370799762)       (1.073074779)       (1.459466579)

  7-17  2.022503185   8-14  2.635902670   9-15  2.566798677   9-16  2.573776414  10-11  2.514696194
       (1.070262671)       (1.394859724)       (1.358291462)       (1.361983922)       (1.330720014)

 10-15  2.590435935  10-24  2.027817297  11-12  2.757991923  11-21  2.022503185  12-16  2.635902670
       (1.370799762)       (1.073074779)       (1.459466579)       (1.070262671)       (1.394859724)

 13-18  1.900377812  14-19  1.884443977  15-22  1.900377812  16-23  1.884443977
       (1.005636703)       (0.997204880)       (1.005636703)       (0.997204880)

 Bond angles

  1--5-13  123.07577386   1--5-14  122.05094466   2--8--7  126.20486319   2--8-14  120.19224842

  3--9-15  123.07577386   3--9-16  122.05094466   4-12-11  126.20486319   4-12-16  120.19224842

  5-13--6  122.44197750   5-13-18  116.62358688   5-14--8  127.35121966   5-14-19  116.07821742

  6--7--8  119.10219759   6--7-17  122.49754050   6-13-18  120.93443562   7--6-13  122.62843538

  7--6-20  122.62073131   7--8-14  113.60288839   8--7-17  118.40026191   8-14-19  116.57056292

  9-15-10  122.44197750   9-15-22  116.62358688   9-16-12  127.35121966   9-16-23  116.07821742

 10-11-12  119.10219759  10-11-21  122.49754050  10-15-22  120.93443562  11-10-15  122.62843538

 11-10-24  122.62073131  11-12-16  113.60288839  12-11-21  118.40026191  12-16-23  116.57056292

 13--5-14  114.87328149  13--6-20  114.75083331  15--9-16  114.87328149  15-10-24  114.75083331

 NUCLEAR CHARGE:                   58
 NUMBER OF PRIMITIVE AOS:         480
 NUMBER OF SYMMETRY AOS:          464
 NUMBER OF CONTRACTIONS:          240   ( 176A'  +  64A"  )
 NUMBER OF CORE ORBITALS:           8   (   8A'  +   0A"  )
 NUMBER OF VALENCE ORBITALS:       36   (  28A'  +   8A"  )


 NUCLEAR REPULSION ENERGY  360.46121681


 Eigenvalues of metric

         1 0.112E-03 0.113E-03 0.407E-03 0.422E-03 0.505E-03 0.546E-03 0.792E-03 0.798E-03
         2 0.112E-01 0.118E-01 0.196E-01 0.208E-01 0.285E-01 0.294E-01 0.302E-01 0.306E-01
 

 Contracted 2-electron integrals neglected if value below      1.0D-11
 AO integral compression algorithm  1   Integral accuracy      1.0D-11

     419.955 MB (compressed) written to integral file ( 29.2%)

     Node minimum: 50.332 MB, node maximum: 56.099 MB
 

 NUMBER OF SORTED TWO-ELECTRON INTEGRALS:   27591744.     BUFFER LENGTH:  32768
 NUMBER OF SEGMENTS:   2  SEGMENT LENGTH:   15956472      RECORD LENGTH: 524288

 Memory used in sort:      16.51 MW

 SORT1 READ  179622569. AND WROTE   13095750. INTEGRALS IN   39 RECORDS. CPU TIME:    16.14 SEC, REAL TIME:    16.81 SEC
 SORT2 READ  105057693. AND WROTE  220672156. INTEGRALS IN 1600 RECORDS. CPU TIME:     1.79 SEC, REAL TIME:     2.24 SEC

 Node minimum:   27576295.  Node maximum:   27591744. integrals

 OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000    0.000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        4.44       601      700      960      900      500      950      970     1001     1100     1400   
                                        BASINP    GEOM    ABASIS   SYMINP     VAR     ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
              2       4        0.71       700     1000     2100     1001   
                                         GEOM     BASIS     RHF     BASIS   
 
 PROGRAMS   *        TOTAL       INT    HF-SCF       INT
 CPU TIMES  *        33.21     30.67      0.27      2.04
 REAL TIME  *        34.96 SEC
 DISK USED  *         1.74 GB
 GA USED    *         0.02 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************

1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner


 NUMBER OF ELECTRONS:      29+   29-    SPACE SYMMETRY=1    SPIN SYMMETRY=Singlet 
 CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
 MAX. NUMBER OF ITERATIONS:       60
 INTERPOLATION TYPE:            DIIS
 INTERPOLATION STEPS:              2 (START)      1 (STEP)
 LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN) 



 
 Molecular orbitals read from record     2100.2  Type=RHF/CANONICAL (state 1.1)
 
 Present basis size:     176  64
 Previous basis size:     72  16
 Previous occupation:     24   5
 Previous closed-shells:  24   5
 Previous core-orbitals:   8   0
 Present occupation:      24   5
 Present closed-shells:   24   5
 Present core-orbitals:    8   0
 Wavefunction symmetry:    1   Singlet 

 Orbital overlap <old|new>:  < 1.1| 1.1> = 0.999845   < 2.1| 2.1> = 0.999845   < 3.1| 3.1> = 0.999840   < 4.1| 4.1> = 0.999840
                             < 5.1| 5.1> = 0.999834   < 6.1| 6.1> = 0.999834   < 7.1| 7.1> = 0.999833   < 8.1| 8.1> = 0.999834
                             < 9.1| 9.1> = 0.999877   <10.1|10.1> = 0.999831   <11.1|11.1> = 0.999872   <12.1|12.1> = 0.999885
                             <13.1|13.1> = 0.999785   <14.1|14.1> = 0.999581   <15.1|15.1> = 0.999438   <16.1|16.1> = 0.999389
                             <17.1|17.1> = 0.999213   <18.1|18.1> = 0.999399   <19.1|19.1> = 0.998827   <20.1|20.1> = 0.999019
                             <21.1|21.1> = 0.998317   <22.1|22.1> = 0.998051   <23.1|23.1> = 0.997233   <24.1|24.1> = 0.996915
                             < 1.2| 1.2> = 0.998237   < 2.2| 2.2> = 0.997922   < 3.2| 3.2> = 0.997883   < 4.2| 4.2> = 0.996161
                             < 5.2| 5.2> = 0.997374
 
 Molecular orbital dump at record        2101.2

 ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.            DIPOLE MOMENTS         DIIS
    1      0.000D+00      0.000D+00      -411.73073285   1017.473241  -1.079271   0.460424   0.000000    0
    2      0.000D+00      0.121D-01      -412.28959118   1006.414508  -1.198336   0.477557   0.000000    1
    3      0.349D-01      0.304D-02      -412.33088507   1008.644703  -1.793587   0.665543   0.000000    2
    4      0.522D-02      0.178D-02      -412.34239904   1008.106571  -1.685578   0.642074   0.000000    3
    5      0.222D-02      0.411D-03      -412.34385235   1007.636796  -1.758609   0.663898   0.000000    4
    6      0.841D-03      0.203D-03      -412.34417766   1007.800518  -1.780726   0.670634   0.000000    5
    7      0.358D-03      0.672D-04      -412.34424380   1007.790212  -1.788627   0.678157   0.000000    6
    8      0.175D-03      0.235D-04      -412.34424983   1007.778300  -1.791681   0.678159   0.000000    7
    9      0.513D-04      0.640D-05      -412.34425031   1007.780701  -1.791832   0.679636   0.000000    8
   10      0.168D-04      0.191D-05      -412.34425033   1007.781129  -1.791908   0.679482   0.000000    8
   11      0.283D-05      0.660D-06      -412.34425034   1007.780879  -1.791927   0.679692   0.000000    0
 
 Final occupancy:  24   5

 !RHF STATE 1.1 ENERGY               -412.34425034
 Nuclear energy                       360.46121681
 One-electron energy                -1276.69590670
 Two-electron energy                  503.89043955
 Virial quotient                       -0.99967323
 !RHF STATE 1.1 DIPOLE MOMENTS:        -1.79192731     0.67969153     0.00000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        4.49       601      700      960      900      500      950      970     1001     1100     1400   
                                        BASINP    GEOM    ABASIS   SYMINP     VAR     ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER   
 
              2       5        1.44       700     1000     2100     1001     2101   
                                         GEOM     BASIS     RHF     BASIS     RHF  
 
 PROGRAMS   *        TOTAL    HF-SCF       INT    HF-SCF       INT
 CPU TIMES  *        42.48      9.26     30.67      0.27      2.04
 REAL TIME  *        44.52 SEC
 DISK USED  *         1.78 GB
 GA USED    *         0.14 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************


1PROGRAM * CCSD (Closed-shell coupled cluster)     Authors: C. Hampel, H.-J. Werner, 1991, M. Deegan, P.J. Knowles, 1992


 Convergence thresholds:  THRVAR = 1.00D-10  THRDEN = 1.00D-06

 CCSD(T)     terms to be evaluated (factor= 1.000)


 Number of core orbitals:           8 (   8   0 )
 Number of closed-shell orbitals:  21 (  16   5 )
 Number of external orbitals:     211 ( 152  59 )

 Setting scratch file implementation to df  

 
 Molecular orbitals read from record     2101.2  Type=RHF/CANONICAL (state 1.1)

 Number of N-1 electron functions:              21
 Number of N-2 electron functions:             231
 Number of singly external CSFs:              2727
 Number of doubly external CSFs:           5172288
 Total number of CSFs:                     5175016

 Length of J-op  integral file:      0.00 MB
 Length of K-op  integral file:      2.19 MB
 Length of 3-ext integral record:    0.00 MB

 Integral transformation finished. Total CPU:  46.92 sec, npass=  1  Memory used:  54.22 MW

 Reference energy:                   -412.34425034
 MP2 correlation energy:               -0.94169647
 MP2 total energy:                   -413.28594681

 ITER.       NORM       CORR.ENERGY   TOTAL ENERGY   ENERGY CHANGE        DEN1      VAR(S)    VAR(P)  DIIS     TIME
   1      1.34028313    -0.92687038  -413.27112072     0.01482609    -0.03489320  0.13D-01  0.67D-02  0  0    83.93
   2      1.36965111    -0.95396677  -413.29821711    -0.02709639    -0.00370343  0.41D-03  0.13D-02  0  0   120.97
   3      1.38122775    -0.95861720  -413.30286754    -0.00465043    -0.00081387  0.35D-03  0.19D-03  1  1   158.19
   4      1.39247947    -0.96420314  -413.30845348    -0.00558594    -0.00012236  0.27D-04  0.43D-04  2  2   195.42
   5      1.39552028    -0.96475542  -413.30900576    -0.00055227    -0.00001158  0.57D-05  0.29D-05  3  3   233.06
   6      1.39647607    -0.96478178  -413.30903211    -0.00002636    -0.00000112  0.53D-06  0.30D-06  4  4   270.84
   7      1.39670475    -0.96483081  -413.30908115    -0.00004903    -0.00000019  0.86D-07  0.52D-07  5  5   308.33
   8      1.39677634    -0.96484101  -413.30909135    -0.00001020    -0.00000002  0.11D-07  0.54D-08  6  6   346.16
   9      1.39677758    -0.96483723  -413.30908756     0.00000379    -0.00000000  0.27D-08  0.11D-08  6  1   383.99
  10      1.39678088    -0.96483834  -413.30908868    -0.00000111    -0.00000000  0.91D-09  0.26D-09  6  2   421.75
  11      1.39677979    -0.96483730  -413.30908763     0.00000104    -0.00000000  0.14D-09  0.46D-10  6  3   459.39
  12      1.39678032    -0.96483773  -413.30908806    -0.00000043    -0.00000000  0.31D-10  0.13D-10  6  4   497.39

 Norm of t1 vector:      0.02667315      S-energy:     0.00000070      T1 diagnostic:  0.01781958
 Norm of t2 vector:      0.37010717      P-energy:    -0.96483843

 Memory could be reduced to 131.8 Mword without degradation in triples

 CPU time for triples:    695.62 sec


 RESULTS
 =======
 !CCSD ENERGY                        -413.309088063363
 !CCSD[T] ENERGY                     -413.354086904032     (Triples contribution  -0.04499884)
 !CCSD-T ENERGY                      -413.348767932089     (Triples contribution  -0.03967987)

 Reference energy                    -412.344250337239
 Correlation energy                    -1.005863671635
 !CCSD(T) ENERGY                     -413.350114008875     (Triples contribution  -0.04102595)

 Program statistics:

 Available memory in ccsd:               474999018
 Min. memory needed in ccsd:              12631341
 Max. memory used in ccsd:                17432123
 Max. memory used in cckext:              16616250 (12 integral passes)



 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      19      505.56       601      700      960      900      500      950      970     1001     1100     1400   
                                        BASINP    GEOM    ABASIS   SYMINP     VAR     ZMAT    AOBASIS   BASIS      S        T 
                                         1410     1200     1210     1080     1600      129     1650     1700     1380   
                                           V       H0       H01     AOSYM     SMH      P2S    MOLCAS    OPER     JKOP   
 
              2       5        1.44       700     1000     2100     1001     2101   
                                         GEOM     BASIS     RHF     BASIS     RHF  
 
 PROGRAMS   *        TOTAL   CCSD(T)    HF-SCF       INT    HF-SCF       INT
 CPU TIMES  *      1235.52   1193.03      9.26     30.67      0.27      2.04
 REAL TIME  *      1331.35 SEC
 DISK USED  *        12.72 GB
 GA USED    *         0.14 MB (max)       0.00 MB (current)
 **********************************************************************************************************************************

        CCSD(T)         HF-SCF          HF-SCF  
   -413.35011401   -412.34425034   -407.07625644
 **********************************************************************************************************************************
 Variable memory released


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