[molpro-user] problem with excited states via CIS

Seth Olsen s.olsen1 at uq.edu.au
Mon Sep 11 10:00:12 BST 2006


Hi Molpro-users,

Thank you for the reponses.  I seems to work now, but I have had no luck 
requesting properties or density matrices for CIS excited states.  Are 
these not coded at this time?

Cheers,

Seth

H. -J. Werner wrote:
> CIS is a command, not a directive of hf. Thus, your input should read
>
>  {hf
>  wf,100,1,0
>  save,2101.2}
>  cis,-10,trans=1
>
> H.-J. Werner
>
>
> On Mo, 11 Sep 2006, Seth Olsen wrote:
>
>   
>> Hi Molpro-Users,
>>
>> I am having trouble with the new Configuration-Interaction facility in 
>> Molpro2006.  I add the CIS command to the HF deck as instructed to do in 
>> the manual, and I the job crashes with the following error:
>>
>> Unknown directive CIS for command HF-SCF
>>
>> GA ERROR checkinp on processor   0
>>
>> Is there a bug in this version?  Is there a patch needed to use CIS 
>> under HF?
>>
>> I have attached the relevant output file (it isn't long).
>>
>> Cheers,
>>
>> Seth
>>
>>
>>
>>     
>
>   
>> MPP nodes  nproc
>> ac44         8
>> ga_uses_ma=false, calling ma_init with nominal heap.
>> GA-space will be limited to   8.0 MW (determined by -G option)
>>
>> Primary working directories:    /jobfs/m03/49580.ac-pbs
>> Secondary working directories:  /jobfs/m03/49580.ac-pbs
>> Working directories for file 2: /short/m03/Melanins/DHICA/cis
>>
>> CPU=
>>  1600.000000:1600.000000:1600.000000:1600.000000:1600.000000:1600.000000:1600.0
>> 00000:1600.000000:1600.000000:1600.000000 MHz
>> Using default tuning parameters for linux_unknown
>>
>> MPP tuning parameters: Latency=     0 Microseconds,   Broadcast speed=    0 MB/sec
>> default implementation of scratch files=sf  
>>
>> ***,DHICA a13 fully protonated;
>> Memory,90,m;
>> file,1,dhica-a13-cis10-dzp.int,new
>> file,2,dhica-a13-cis10-dzp.wfn,new
>> punch,dhica-a13-cis10-dzp.pun
>> Gprint,basis,civector,orbitals,angles=-1,distances=-1;                          ! Print basis information
>>  
>>                                                                                 !Variables :
>> cn2   =     1.38237714
>> cc3   =     1.39480959
>> ccn3  =   108.39880311
>> cc4   =     2.63122458
>> ccc4  =   129.76049036
>> dih4  =    -0.01137429
>> cc5   =     1.39358745
>> ccc5  =   141.49296286
>> dih5  =     0.00000000
>> cc6   =     1.42033882
>> ccc6  =   122.19808127
>> dih6  =     0.00647498
>> cc7   =     1.39440519
>> ccc7  =   120.64790982
>> dih7  =     0.00000000
>> cc8   =     1.41054503
>> ccc8  =   117.60124626
>> dih8  =     0.00000000
>> cc9   =     1.41997566
>> ccc9  =   118.67716795
>> dih9  =     0.00180844
>> oc10  =     1.40596679
>> occ10 =   123.74338997
>> dih10 =   180.00000000
>> oc11  =     1.39008332
>> occ11 =   119.90163893
>> dih11 =   180.00000000
>> cc12  =     1.52872101
>> ccc12 =   134.29105112
>> dih12 =  -179.99305437
>> oc13  =     1.26210722
>> occ13 =   116.14467651
>> dih13 =     0.03641154
>> oc14  =     1.27535339
>> occ14 =   112.86209409
>> dih14 =   180.04415907
>> hc15  =     1.08553053
>> hcc15 =   128.54275756
>> dih15 =     0.00000000
>> hc16  =     1.09471473
>> hcc16 =   120.90887394
>> dih16 =   179.99850231
>> hc17  =     1.09100577
>> hcc17 =   122.80612189
>> dih17 =   179.99738061
>> hn18  =     1.01979413
>> hnc18 =   131.04872629
>> dih18 =     0.01390361
>> ho19  =     0.97295714
>> hoc19 =   107.50130672
>> dih19 =     0.00963956
>> ho20  =     0.97603429
>> hoc20 =   105.93458957
>> dih20 =  -180.00291726
>>  
>> geometry={NOSYM;NOORIENT;ANGSTROM;
>>                                                                             ! geometry input in Z-MATRIX type generated by gabedit
>> N;
>> C,1,cn2;
>> C,2,cc3,1,ccn3;
>> C,3,cc4,2,ccc4,1,dih4;
>> C,4,cc5,3,ccc5,2,dih5;
>> C,5,cc6,4,ccc6,3,dih6;
>> C,6,cc7,5,ccc7,4,dih7;
>> C,7,cc8,6,ccc8,5,dih8;
>> C,4,cc9,5,ccc9,6,dih9;
>> O,5,oc10,4,occ10,9,dih10;
>> O,6,oc11,7,occ11,8,dih11;
>> C,2,cc12,3,ccc12,9,dih12;
>> O,12,oc13,2,occ13,3,dih13;
>> O,12,oc14,2,occ14,3,dih14;
>> H,3,hc15,9,hcc15,4,dih15;
>> H,4,hc16,9,hcc16,8,dih16;
>> H,7,hc17,8,hcc17,9,dih17;
>> H,1,hn18,8,hnc18,7,dih18;
>> H,10,ho19,5,hoc19,4,dih19;
>> H,11,ho20,6,hoc20,7,dih20;
>> }
>> Including file /home/564/sco564/Basis-Sets/Dunning-DZP.txt
>>  
>> {hf
>> wf,100,1,0
>> save,2101.2
>> cis,-10,trans=1}
>>  
>> {matrop
>> load,orbitals,orb,2101.2
>> write,orbitals,dhica-a13-cis10-dzp.orb}
>>  
>> pop;density,2101.2,state=1.1
>> pop;density,2101.2,state=2.1
>> pop;density,2101.2,state=3.1
>> pop;density,2101.2,state=4.1
>> pop;density,2101.2,state=5.1
>> pop;density,2101.2,state=6.1
>> pop;density,2101.2,state=7.1
>> pop;density,2101.2,state=8.1
>> pop;density,2101.2,state=9.1
>> pop;density,2101.2,state=10.1
>>  
>> cube,dhica-a13-cis10-dzp-s0.cube;density,2101.2,state=1.1
>> cube,dhica-a13-cis10-dzp-s1.cube;density,2101.2,state=2.1
>> cube,dhica-a13-cis10-dzp-s2.cube;density,2101.2,state=3.1
>> cube,dhica-a13-cis10-dzp-s3.cube;density,2101.2,state=4.1
>> cube,dhica-a13-cis10-dzp-s4.cube;density,2101.2,state=5.1
>> cube,dhica-a13-cis10-dzp-s5.cube;density,2101.2,state=6.1
>> cube,dhica-a13-cis10-dzp-s6.cube;density,2101.2,state=7.1
>> cube,dhica-a13-cis10-dzp-s7.cube;density,2101.2,state=8.1
>> cube,dhica-a13-cis10-dzp-s8.cube;density,2101.2,state=9.1
>> cube,dhica-a13-cis10-dzp-s9.cube;density,2101.2,state=10.1
>>  
>> put,molden,dhica-a13-cis10-dzp.molden
>>  
>>  
>>
>> Variables initialized (516), CPU time= 0.01 sec
>> Commands  initialized (293), CPU time= 0.02 sec, 434 directives.
>> Default parameters read. Elapsed time= 0.08 sec
>> Checking input...
>>
>> Unknown directive CIS for command HF-SCF
>>
>> GA ERROR checkinp on processor   0                                       
>>     
>
>
>   




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