[molpro-user] A question about density-fitting in SAPT

cong.wang cong.wang at helsinki.fi
Fri May 8 16:15:10 BST 2009


Dear Dr. Hesselmann,

  Many thanks for your reply. If I do a DF-DFT-SAPT calculation for
He2, what is the correct input format? I feel molpro is quite
sensitive for the format. If the input like

*********************
r=5.6
 geometry={nosym; he1; he2,he1,r}
 basis=avqz


          !wf records
 ca=2101.2
 cb=2102.2



          !monomer A
 dummy,he2
 {ks,pbe;asymp,0.324; save,$ca}
 sapt;monomerA


          !monomer B
 dummy,he1
 {ks,pbe;asymp,0.324; start,atdens; save,$cb}
 sapt;monomerB


          !interaction contributions
 sapt;intermol,ca=$ca,cb=$cb
******************************

how to combine with
***************
{sapt;intermol,ca=$ca,cb=$cb,fitlevel=3
dfit,basis_coul=jkfit,basis_exch=jkfit,basis_mp2=mp2fit,cfit_scf=3}
*******************************

The He2 is a testing case for some big system, therefore the
density-fitting is necessary for further calculation.

Best regards
Cong Wang

Department of Chemistry
Laboratory for Instruction in Swedish
University of Helsinki
A.I. Virtanens plats 1
P.O. Box 55
FI-00014 University of Helsinki
FINLAND



2009/5/7 Andreas Hesselmann <andreas.hesselmann at chemie.uni-erlangen.de>:
> Dear Cong,
>
> the problem with your input is that you try to
> do a df-dft-sapt calculation with Hartree-Fock
> monomer orbitals. This is not supported
> (at the moment), but you have several options
> to fix this:
>
> 1) still do hf/df-dft-sapt by calculating
>   the integration grid in advance:
>   insert
>         {grid}
>   in your input (see also the testjobs
>   by the way). Note, however, that then
>   your results will not be meaningful
>   because you combine the nonlocal-exchange
>   potential (hf) with a local xc-kernel
>   (alda).
>
> 2) do a (non-hybrid)dft/df-dft-sapt calculation,
>   i.e. instead of calculating the monomer orbitals
>   with Hartree-Fock, calculate them with some
>   'proper' DFT-functional (see manual for more
>   information about this method).
>
> 3) The dimer you intend to investigate is very small,
>   so you don't need to use density-fitting at all,
>   in fact the conventional sapt could in this case
>   be even faster. Then you can do full hf-sapt calcs,
>   see testjob 'near_hfsapt' for an example input.
>
> Wishes,
> Andreas
>
>
> On Wednesday 06 May 2009 20:04, cwang at mappi.helsinki.fi wrote:
>> Dear Dr. Hill.
>>
>>    Hi,
>>
>>    Many thanks for your suggestion, now it seems work, but, the outout ends
>> at
>>
>> " ? Error
>>   ? Record not found
>>   ? The problem occurs in readm
>>
>>   ERROR EXIT
>>   CURRENT STACK:      GRID_COMPUTE  MAIN
>> "
>>
>> What is the reason for that and how to fix this problem?
>>
>> Here is the whole output file
>> Thank you very much
>> Best regards
>> Cong Wang
>>
>> *********************
>>   CPU=Opteron 2400.358:2400.358:2400.358:2400.358 MHz
>>   mxmblk= 64  mxmbln= 64  ncache=  16384  mindgm= 11  mindgv= 33
>> mindgc=  4  mindgl=  4  mindgr=  1  noblas=0  nroll=2  minvec=7
>>   default implementation of scratch files=df
>>
>>   ***,
>>   r=5.6
>>   geometry={nosym; he1; he2,he1,r}
>>   basis={
>>   default,avdz
>>   set,jkfit
>>   s, He, 66.205029000,13.171713600,3.1622361000,0.81536220000
>>   c,1.1, 0.53033986000E-01
>>   c,2.2, 0.39465220220
>>   c,3.3, 0.91729877120
>>   p, He, 9.6128819820,3.2042939700,1.1643102000
>>   d, He, 7.6739799000,0.98779470000
>>
>>   set,mp2fit
>>   default,avdz/mp2fit
>>   }
>>
>>
>>             !wf records
>>   ca=2101.2
>>   cb=2102.2
>>
>>
>>
>>             !monomer A
>>   dummy,he2
>>   {hf; save,$ca}
>>   sapt;monomerA
>>
>>
>>             !monomer B
>>   dummy,he1
>>   {hf; start,atdens; save,$cb}
>>   sapt;monomerB
>>
>>
>>             !interaction contributions
>>   {sapt;intermol,ca=$ca,cb=$cb,fitlevel=3
>>   dfit,basis_coul=jkfit,basis_exch=jkfit,basis_mp2=mp2fit,cfit_scf=3}
>>
>>
>>
>>   Variables initialized (517), CPU time= 0.01 sec
>>   Commands  initialized (293), CPU time= 0.02 sec, 437 directives.
>>   Default parameters read. Elapsed time= 0.07 sec
>>   Checking input...
>>   Passed
>> 1
>>
>>
>>                                           ***  PROGRAM SYSTEM MOLPRO  ***
>>                           Copyright, University College Cardiff
>> Consultants Limited, 2004
>>
>>                                      Version 2006.1 linked 10 Mar 2008
>> 13:07:39
>>
>>
>>
>> ***************************************************************************
>>******************************************************* LABEL *
>>   Linux-2.6.9-42.7sp.XCsmp/c553(x86_64) 64 bit version (path/acml)
>>                     DATE:   6-May-09         TIME: 20:42:36
>>
>> ***************************************************************************
>>*******************************************************
>>
>>   Patch level:      151
>>
>> ***************************************************************************
>>******************************************************* SETTING R
>>   =         5.60000000
>>
>>   Variable memory set to    7272727 words,  buffer space   230000 words
>>
>>   SETTING BASIS          =    AVDZ
>>   SETTING CA             =      2101.20000000
>>   SETTING CB             =      2102.20000000
>>
>>   Dummy atoms: HE2
>>
>>
>>   Recomputing integrals since basis changed
>>
>>
>>   Using spherical harmonics
>>
>>   Library entry HE     S aug-cc-pVDZ          selected for orbital group  1
>>   Library entry HE     P aug-cc-pVDZ          selected for orbital group  1
>>
>> 1PROGRAM * SEWARD (Integral evaluation for generally contracted
>> gaussian basis sets)     Author: Roland Lindh, 1990
>>
>>   Geometry written to block  1 of record 700
>>
>>   Orientation using atomic masses
>>   Molecule type: Linear
>>   Rotational constants:      28.7558807     28.7558807      0.0000000 GHz
>>
>>   Point group  C1
>>
>>
>>
>>   ATOMIC COORDINATES
>>
>>   NR  ATOM    CHARGE       X              Y              Z
>>
>>     1  HE1     2.00    0.000000000    0.000000000   -2.800000000
>>     2  HE2     0.00    0.000000000    0.000000000    2.800000000
>>
>>   Bond lengths in Bohr (Angstrom)
>>
>>   1-2  5.600000000
>>       (2.963392594)
>>
>>   NUCLEAR CHARGE:                    2
>>   NUMBER OF PRIMITIVE AOS:          22
>>   NUMBER OF SYMMETRY AOS:           22
>>   NUMBER OF CONTRACTIONS:           18   (  18A   )
>>   NUMBER OF CORE ORBITALS:           0   (   0A   )
>>   NUMBER OF VALENCE ORBITALS:        1   (   1A   )
>>
>>
>>   NUCLEAR REPULSION ENERGY    0.00000000
>>
>>   EXTRA SYMMETRY OF AOS IN SYMMETRY 1:   1 1 1 2 3 1 2 3 1 1   1 1 2 3 1 2
>> 3 1
>>
>>   Eigenvalues of metric
>>
>>           1 0.722E-01 0.778E-01 0.311E+00 0.507E+00 0.523E+00
>> 0.523E+00 0.532E+00 0.542E+00
>>
>>
>>   Contracted 2-electron integrals neglected if value below      1.0E-11
>>
>>   Basis set:  JKFIT
>>   Basis size:   46
>>   Attributes:
>>   Sphericals:   T
>>   Library entry HE     S aug-cc-pVDZ-MP2F     selected for MP2FIT group  1
>>   Library entry HE     P aug-cc-pVDZ-MP2F     selected for MP2FIT group  1
>>   Basis set:  MP2FIT
>>   Basis size:   26
>>   Attributes:
>>   Sphericals:   T
>>
>>
>> ***************************************************************************
>>*******************************************************
>>
>>   AO integral compression algorithm  1   Integral accuracy      1.0E-11
>>
>>       0.262 MB (compressed) written to integral file ( 42.1%)
>>
>>
>>   NUMBER OF SORTED TWO-ELECTRON INTEGRALS:      14706.     BUFFER
>> LENGTH:  32768
>>   NUMBER OF SEGMENTS:   1  SEGMENT LENGTH:      14706      RECORD
>> LENGTH: 524288
>>
>>   Memory used in sort:       0.57 MW
>>
>>   SORT1 READ      26487. AND WROTE       4241. INTEGRALS IN    1
>> RECORDS. CPU TIME:     0.00 SEC, REAL TIME:     0.05 SEC
>>   SORT2 READ       4241. AND WROTE      14706. INTEGRALS IN    1
>> RECORDS. CPU TIME:     0.01 SEC, REAL TIME:     0.03 SEC
>>
>>   FILE SIZES:   FILE 1:    2.0 MBYTE,  FILE 4:    4.2 MBYTE,   TOTAL:
>>    6.3 MBYTE
>>
>>   OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000
>>     0.000000
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>   PROGRAMS   *        TOTAL       INT
>>   CPU TIMES  *         0.21      0.06
>>   REAL TIME  *        20.42 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>> 1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner
>>
>>
>>   NUMBER OF ELECTRONS:       1+    1-
>>   CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
>>   MAX. NUMBER OF ITERATIONS:       60
>>   INTERPOLATION TYPE:            DIIS
>>   INTERPOLATION STEPS:              2 (START)      1 (STEP)
>>   LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN)
>>
>>
>>
>>   Orbital guess generated from atomic densities.  Occupancy:    1
>>
>>   Molecular orbital dump at record        2101.2
>>
>>   ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.
>>            DIPOLE MOMENTS         DIIS
>>      1      0.000E+00      0.000E+00        -2.85568404      2.045930
>>   0.000000   0.000000  -0.000208    0
>>      2      0.000E+00      0.552E-03        -2.85571088      2.043679
>>   0.000000   0.000000  -0.000305    1
>>      3      0.809E-03      0.124E-03        -2.85571232      2.043002
>>   0.000000   0.000000  -0.000340    2
>>      4      0.237E-03      0.768E-06        -2.85571233      2.043002
>>   0.000000   0.000000  -0.000342    3
>>      5      0.904E-06      0.520E-07        -2.85571233      2.043002
>>   0.000000   0.000000  -0.000342    0
>>
>>   Final occupancy:   1
>>
>>   !RHF STATE 1.1 ENERGY                 -2.855712325032
>>   Nuclear energy                         0.00000000
>>   One-electron energy                   -3.87721318
>>   Two-electron energy                    1.02150086
>>   Virial quotient                       -1.00362394
>>   !RHF STATE 1.1 DIPOLE MOMENT           0.00000000     0.00000000
>> -0.00034186
>>   Dipole moment /Debye                   0.00000000     0.00000000
>> -0.00086887
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>                2       3        0.26       700     1000     2101
>>                                           GEOM     BASIS     RHF
>>
>>   PROGRAMS   *        TOTAL        HF       INT
>>   CPU TIMES  *         0.22      0.01      0.06
>>   REAL TIME  *        22.52 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>>   PROGRAM * SAPT
>>   Fix monomer properties
>>
>>   Geometry for monomer A:
>>      1
>>   HE   2.00      0.00000000      0.00000000     -2.80000000
>>   Nuclear attraction integrals written to record:     1001.3
>>   Occupied orbitals of monomer A:     1
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>                2       3        0.26       700     1000     2101
>>                                           GEOM     BASIS     RHF
>>
>>   PROGRAMS   *        TOTAL      SAPT        HF       INT
>>   CPU TIMES  *         0.22      0.00      0.01      0.06
>>   REAL TIME  *        22.66 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>>   Dummy atoms: HE1
>>
>>
>>   Recomputing one-electron integrals since nuclear charges changed
>>
>> 1PROGRAM * SEWARD (Integral evaluation for generally contracted
>> gaussian basis sets)     Author: Roland Lindh, 1990
>>
>>   Geometry written to block  1 of record 700
>>
>>   Orientation using atomic masses
>>   Molecule type: Linear
>>   Rotational constants:      28.7558807     28.7558807      0.0000000 GHz
>>
>>   Point group  C1
>>
>>
>>
>>   ATOMIC COORDINATES
>>
>>   NR  ATOM    CHARGE       X              Y              Z
>>
>>     1  HE1     0.00    0.000000000    0.000000000   -2.800000000
>>     2  HE2     2.00    0.000000000    0.000000000    2.800000000
>>
>>   Bond lengths in Bohr (Angstrom)
>>
>>   1-2  5.600000000
>>       (2.963392594)
>>
>>   NUCLEAR CHARGE:                    2
>>   NUMBER OF PRIMITIVE AOS:          22
>>   NUMBER OF SYMMETRY AOS:           22
>>   NUMBER OF CONTRACTIONS:           18   (  18A   )
>>   NUMBER OF CORE ORBITALS:           0   (   0A   )
>>   NUMBER OF VALENCE ORBITALS:        1   (   1A   )
>>
>>   MOLECULE CHANGED: INITIALIZING OCCUPATION AND DUMP RECORDS
>>
>>
>>   NUCLEAR REPULSION ENERGY    0.00000000
>>
>>   EXTRA SYMMETRY OF AOS IN SYMMETRY 1:   1 1 1 2 3 1 2 3 1 1   1 1 2 3 1 2
>> 3 1
>>
>>   Eigenvalues of metric
>>
>>           1 0.722E-01 0.778E-01 0.311E+00 0.507E+00 0.523E+00
>> 0.523E+00 0.532E+00 0.542E+00
>>
>>
>>   Contracted 2-electron integrals neglected if value below      1.0E-11
>>   Basis set:  JKFIT
>>   Basis size:   46
>>   Attributes:
>>   Sphericals:   T
>>   Library entry HE     S aug-cc-pVDZ-MP2F     selected for MP2FIT group  1
>>   Library entry HE     P aug-cc-pVDZ-MP2F     selected for MP2FIT group  1
>>   Basis set:  MP2FIT
>>   Basis size:   26
>>   Attributes:
>>   Sphericals:   T
>>
>>   OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000
>>     0.000000
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>                2       3        0.26       700     1000     2101
>>                                           GEOM     BASIS     RHF
>>
>>   PROGRAMS   *        TOTAL       INT      SAPT        HF       INT
>>   CPU TIMES  *         0.26      0.04      0.00      0.01      0.06
>>   REAL TIME  *        22.76 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>> 1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner
>>
>>
>>   NUMBER OF ELECTRONS:       1+    1-
>>   CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
>>   MAX. NUMBER OF ITERATIONS:       60
>>   INTERPOLATION TYPE:            DIIS
>>   INTERPOLATION STEPS:              2 (START)      1 (STEP)
>>   LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN)
>>
>>
>>
>>   Orbital guess generated from atomic densities.  Occupancy:    1
>>
>>   Molecular orbital dump at record        2102.2
>>
>>   ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.
>>            DIPOLE MOMENTS         DIIS
>>      1      0.000E+00      0.000E+00        -2.85568404      2.045930
>>   0.000000   0.000000   0.000208    0
>>      2      0.000E+00      0.552E-03        -2.85571088      2.043679
>>   0.000000   0.000000   0.000305    1
>>      3      0.809E-03      0.124E-03        -2.85571232      2.043002
>>   0.000000   0.000000   0.000340    2
>>      4      0.237E-03      0.768E-06        -2.85571233      2.043002
>>   0.000000   0.000000   0.000342    3
>>      5      0.904E-06      0.520E-07        -2.85571233      2.043002
>>   0.000000   0.000000   0.000342    0
>>
>>   Final occupancy:   1
>>
>>   !RHF STATE 1.1 ENERGY                 -2.855712325032
>>   Nuclear energy                         0.00000000
>>   One-electron energy                   -3.87721318
>>   Two-electron energy                    1.02150086
>>   Virial quotient                       -1.00362394
>>   !RHF STATE 1.1 DIPOLE MOMENT           0.00000000     0.00000000
>> 0.00034186
>>   Dipole moment /Debye                   0.00000000     0.00000000
>> 0.00086887
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>                2       4        0.31       700     1000     2101     2102
>>                                           GEOM     BASIS     RHF      RHF
>>
>>   PROGRAMS   *        TOTAL        HF       INT      SAPT        HF
>> INT CPU TIMES  *         0.27      0.01      0.04      0.00      0.01
>> 0.06 REAL TIME  *        22.78 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>>   PROGRAM * SAPT
>>   Fix monomer properties
>>
>>   Geometry for monomer B:
>>      1
>>   HE   2.00      0.00000000      0.00000000      2.80000000
>>   Nuclear attraction integrals written to record:     1002.3
>>   Occupied orbitals of monomer B:     1
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      19        1.80       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>
>>                2       4        0.31       700     1000     2101     2102
>>                                           GEOM     BASIS     RHF      RHF
>>
>>   PROGRAMS   *        TOTAL      SAPT        HF       INT      SAPT
>>      HF       INT
>>   CPU TIMES  *         0.27      0.00      0.01      0.04      0.00
>>    0.01      0.06
>>   REAL TIME  *        22.78 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>>
>>   PROGRAM * SAPT      Authors: A. Hesselmann, G. Jansen, 2003
>>
>>   (Calculation of intermolecular interaction energy contributions
>>    for single-determinant wave-functions)
>>
>>   Monomer A wave function in record             2101.2
>>   Monomer A electrostatic potential in record   1001.3
>>   Monomer B wave function in record             2102.2
>>   Monomer B electrostatic potential in record   1002.3
>>   Overlap matrix in record                      1000.3
>>
>>   Factor for nonlocal exchange:    1.000000
>>   Print factor:   0
>>   Density fitting level:   3
>>   Level of calculation:    3
>>
>>   CPKS solver:    1
>>   CPKS convergence threshold:   0.10000000E-05
>>   CPKS maximumb number of iterations:     50
>>
>>   Occupied space for monomer A:    1
>>   Virtual  space for monomer A:   17
>>
>>   Occupied space for monomer B:    1
>>   Virtual  space for monomer B:   17
>>
>>   Memory available:                             7272627 words
>>   Approximate memory needed for E2disp:           11276 words
>>   Approximate memory needed for E2exch-disp:      11403 words
>>
>>
>>   Transform atomic integrals
>>   ==========================
>>   J/K matrices for monomer A
>>   J/K matrices for monomer B
>>   W matrix for monomer A
>>   W matrix for monomer B
>>
>>   CPU time for integrals:       0.11 sec
>>
>>
>>   Response calculations
>>   ---------------------
>>   Calculate response for monomer A
>>   ITER    DIFF       Induction     Time
>>     1    0.000282    0.000000      0.00
>>     2    0.000060    0.000000      0.07
>>     3    0.000013    0.000000      0.00
>>     4    0.000001    0.000000      0.01
>>     5    0.000000    0.000000      0.01
>>   Second order induction =      -0.00000041
>>
>>
>>   CPU time for CPKS(A):       0.09 sec
>>
>>   Norm: COULOMB
>>
>>   Computing (ia|fxc|P) integrals...
>>   XC-Kernel density threshold for (ia|fxc|P):  0.10000000E-07
>>   XC-Kernel density threshold for (P|fxc|Q):   0.10000000E-05
>>
>>
>>   FILE 1 RECORD      -1 OFFSET=          1. NOT FOUND
>>
>>   Records on file 1
>>
>>   IREC   NAME  TYPE        OFFSET    LENGTH   IMPLEMENTATION   EXT
>> PREV   PARENT  MPP_STATE
>>     1     500  VAR          4096.    88402.         df          0
>> 0      0      0
>>     2     610  BASINP      92498.     8192.         df          0
>> 0      0      0
>>     3     700  GEOM       100690.    23316.         df          0
>> 0      0      0
>>     4     900  SYMINP     124006.      136.         df          0
>> 0      0      0
>>     5     950  ZMAT       124142.       82.         df          0
>> 0      0      0
>>     6     970  AOBASIS    124224.      147.         df          0
>> 0      0      0
>>     7    1000  BASIS      124371.      688.         df          0
>> 0      0      0
>>     8    1100  S          125059.      173.         df          0
>> 0      0      0
>>     9    1400  T          125232.      173.         df          0
>> 0      0      0
>>    10    1410  V          125405.      173.         df          0
>> 0      0      0
>>    11    1200  H0         125578.      173.         df          0
>> 0      0      0
>>    12    1210  H01        125751.      173.         df          0
>> 0      0      0
>>    13    1080  AOSYM      125924.       26.         df          0
>> 0      0      0
>>    14    1600  SMH        125950.      171.         df          0
>> 0      0      0
>>    15     129  P2S        126121.       48.         df          0
>> 0      0      0
>>    16     960  ABASIS     126169.      463.         df          0
>> 0      0      0
>>    17    1650  MOLCAS     126632.    93950.         df          0
>> 0      0      0
>>    18    1300  ERIS       220582.     4062.         df          0
>> 0      0      0
>>    19    1700  OPER       224644.      553.         df          0
>> 0      0      0
>>    20    2541             225197.      830.         df          0
>> 0      0      0
>>    21    2542             226027.      830.         df          0
>> 0      0      0
>>
>>   ? Error
>>   ? Record not found
>>   ? The problem occurs in readm
>>
>>   ERROR EXIT
>>   CURRENT STACK:      GRID_COMPUTE  MAIN
>>
>>
>>
>> ***************************************************************************
>>******************************************************* DATASETS  * FILE
>> NREC   LENGTH (MB)   RECORD NAMES
>>                1      21        1.81       500      610      700
>> 900      950      970     1000     1100     1400     1410
>>                                            VAR    BASINP    GEOM
>> SYMINP    ZMAT    AOBASIS   BASIS      S        T        V
>>                                           1200     1210     1080
>> 1600      129      960     1650     1300     1700     2541
>>                                            H0       H01     AOSYM
>> SMH      P2S    ABASIS   MOLCAS    ERIS     OPER
>>                                           2542
>>
>>                2       4        0.31       700     1000     2101     2102
>>                                           GEOM     BASIS     RHF      RHF
>>
>>                4       7        0.05      2401     2501     2402
>> 2502     2601     2602     3301
>>                                           J(A)     K(A)     J(B)
>> K(B)     W(A)     W(B)    CPC(A)
>>
>>                5       1        0.04      2543
>>
>>                6       1        0.04      2542
>>
>>   PROGRAMS   *        TOTAL    FEHLER      SAPT        HF       INT
>>    SAPT        HF       INT
>>   CPU TIMES  *         0.48      0.21      0.00      0.01      0.04
>>    0.00      0.01      0.06
>>   REAL TIME  *        26.82 SEC
>>   DISK USED  *         6.71 MB
>>
>> ***************************************************************************
>>*******************************************************
>>
>> Quoting "Grant Hill" <jghill at wsu.edu>:
>> > Cong,
>> >
>> > Try putting your explicit basis definition within the basis block, e.g.
>> >
>> > basis={
>> > default,avdz
>> >
>> > set,jkfit
>> > s, He, 66.205029000,13.171713600,3.1622361000,0.81536220000
>> > c,1.1, 0.53033986000E-01
>> > c,2.2, 0.39465220220
>> > c,3.3, 0.91729877120
>> > p, He, 9.6128819820,3.2042939700,1.1643102000
>> > d, He, 7.6739799000,0.98779470000
>> >
>> > set,mp2fit
>> > default,avdz/mp2fit
>> > }
>> >
>> > HTH,
>> >
>> > Grant
>> >
>> > On 6 May 2009, at 08:03, cwang at mappi.helsinki.fi wrote:
>> >> Glen,
>> >>
>> >>  Hi,
>> >>
>> >>  Many thanks for your reply, I try to add the comma before the
>> >> angular momentum, still the same problem exists, here is the whole
>> >> output file :(
>> >> Sorry for trouble you
>> >>
>> >> Best regards
>> >> Cong
>> >>
>> >> CPU=Opteron 2600.401:2600.401:2600.401:2600.401 MHz
>> >> mxmblk= 64  mxmbln= 64  ncache=  16384  mindgm= 11  mindgv= 33
>> >> mindgc=  4  mindgl=  4  mindgr=  1  noblas=0  nroll=2  minvec=7
>> >> default implementation of scratch files=df
>> >>
>> >> ***,
>> >> r=5.6
>> >> geometry={nosym; he1; he2,he1,r}
>> >> basis={
>> >> default,avdz
>> >> set,jkfit
>> >> default,TM/jkfit
>> >> set,mp2fit
>> >> default,avdz/mp2fit
>> >> }
>> >>
>> >> TM={
>> >> s, HE, 66.205029000,13.171713600,3.1622361000,0.81536220000
>> >> c,1.1, 0.53033986000E-01
>> >> c,2.2, 0.39465220220
>> >> c,3.3, 0.91729877120
>> >> c,4.4, 1.0000000000
>> >> p, HE, 9.6128819820,3.2042939700,1.1643102000
>> >> c,1.1, 1.0000000000
>> >> c,2.2, 1.0000000000
>> >> c,3.3, 1.0000000000
>> >> d, HE, 7.6739799000,0.98779470000
>> >> c,1.1, 1.0000000000
>> >> c,2.2, 1.0000000000
>> >> }
>> >>
>> >>
>> >>
>> >>           !wf records
>> >> ca=2101.2
>> >> cb=2102.2
>> >>
>> >>
>> >>
>> >>           !monomer A
>> >> dummy,he2
>> >> {hf; save,$ca}
>> >> sapt;monomerA
>> >>
>> >>
>> >>           !monomer B
>> >> dummy,he1
>> >> {hf; start,atdens; save,$cb}
>> >> sapt;monomerB
>> >>
>> >>
>> >>           !interaction contributions
>> >> {sapt;intermol,ca=$ca,cb=$cb,fitlevel=3
>> >> dfit,basis_coul=jkfit,basis_exch=jkfit,basis_mp2=mp2fit,cfit_scf=3}
>> >>
>> >>
>> >>
>> >> Variables initialized (517), CPU time= 0.01 sec
>> >> Commands  initialized (293), CPU time= 0.01 sec, 437 directives.
>> >> Default parameters read. Elapsed time= 0.06 sec
>> >> Checking input...
>> >>
>> >> Unknown command or directive S
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive P
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive D
>> >>
>> >> Unknown command or directive C
>> >>
>> >> Unknown command or directive C
>> >>
>> >>   12 input errors found
>> >>
>> >> ? Error
>> >> ? Input errors!
>> >> ? The problem occurs in check_input
>> >>
>> >> ERROR EXIT
>> >> CURRENT STACK:      MAIN
>> >>
>> >>
>> >>
>> >> ************************************************************************
>> >>********************************************************** PROGRAMS   *
>> >>      TOTAL
>> >> CPU TIMES  *         0.14
>> >> REAL TIME  *         0.20 SEC
>> >> DISK USED  *         0.00 MB
>> >>
>> >> ************************************************************************
>> >>**********************************************************
>>
>> _______________________________________________
>> Molpro-user mailing list
>> Molpro-user at molpro.net
>> http://www.molpro.net/mailman/listinfo/molpro-user
>
> --
> --------------------------------------------------
> Andreas Hesselmann
> Institut für Physikalische und Theoretische Chemie
> Universität Erlangen
> Egerlandstraße 3
> 91058 Erlangen / Germany
> Phone:  +49 9131/85-25021
> E-Mail: andreas.hesselmann at chemie.uni-erlangen.de
> -------------------------------------------------
> _______________________________________________
> Molpro-user mailing list
> Molpro-user at molpro.net
> http://www.molpro.net/mailman/listinfo/molpro-user
>



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