[molpro-user] center of charge orientation

Somnath BHOWMICK somnath.bhowmick at etu.univ-amu.fr
Fri Sep 19 17:16:50 BST 2014


Dear Molpro Users,

I am trying to calculate CASSCF energies for an anionic H2+F- system. I am orienting the system such that the origin is set at the center of charge.  At this origin, the dipole moment of the system should vanish. However, the dipole moment obtained in HF and corresponding CASSCF calculation is not zero, and is quite high. 
Any suggestions?

I am attaching the output of my calculation with this mail.

Thanks in advance.

Somnath Bhowmick

-------------- next part --------------

 Primary working directories    : /scratch/ctom.143063
 Secondary working directories  : /scratch/ctom.143063
 Wavefunction directory         : /home/ctom/wfu/
 Main file repository           : /scratch/ctom.143063/

 SHA1      : 49c3320f5d14aae7c3f0c94fbb42bda48d29228e
 ARCHNAME  : Linux/x86_64
 FC        : /opt/intel/composer_xe_2013_sp1.1.106/bin/intel64/ifort
 FCVERSION : 14.0.1
 BLASLIB   : -Wl,-_start-group /opt/intel/mkl/lib/intel64/libmkl_intel_ilp64.a /opt/intel/mkl/lib/intel64/libmkl_sequential.a /opt/intel/mkl/lib/intel64/libmkl_core.a -Wl,-_end-group
 id        : reignier

 Nodes       nprocs
 lame25.crcmm    8
 ga_uses_ma=false, calling ma_init with nominal heap.
 GA-space will be limited to   8.0 MW (determined by -G option)

 Using customized tuning parameters: mindgm=16; mindgv=24; mindgc=8; mindgr=1; noblas=0; minvec=7
 default implementation of scratch files=sf  

    ***, H2F-
     memory,50,M
     gprint,orbitals,civector
 
     ANG
     orient,charge
     symmetry,X,Y
     geometry = {
     dum;
     F dum r1;
     H,dum,rHdum,F,theta;
     H,dum,rHdum,F,180-theta,H,180}
 
     rHH=0.7414
     rHdum=0.5*rHH
     theta=90
     basis=AVQZ
     r1=10.00
 
           {rhf;
           wf,12,1,0
           orbital,2140.2
           }
           {casscf;
           wf,12,1,0
           state,1
           orbital,2141.2,state=1.1}

 Variables initialized (774), CPU time= 0.05 sec
 Commands  initialized (547), CPU time= 0.03 sec, 516 directives.
 Default parameters read. Elapsed time= 0.37 sec

 Checking input...
 Passed
1


                                         ***  PROGRAM SYSTEM MOLPRO  ***
                         Copyright, University College Cardiff Consultants Limited, 2008

                                    Version 2012.1 linked Nov 28 2013 13:33:33


 **********************************************************************************************************************************
 LABEL *                                                                                 
 Linux-2.6.32-431.23.3.el6.x86_64/lame25.crcmm(x86_64) 64 bit mpp version                DATE: 19-Sep-14          TIME: 18:03:04  
 **********************************************************************************************************************************

 SHA1:             49c3320f5d14aae7c3f0c94fbb42bda48d29228e
 **********************************************************************************************************************************


 Variable memory set to   50000000 words,  buffer space   230000 words

 ZSYMEL=X  Y  
 ZCENTRE=CHARGE
 ZUNIT=ANG
 
 SETTING RHH            =         0.74140000                                  
 SETTING RHDUM          =         0.37070000                                  
 SETTING THETA          =        90.00000000                                  
 SETTING BASIS          =    AVQZ
 SETTING R1             =        10.00000000                                  


 Recomputing integrals since basis changed


 Using spherical harmonics

 Library entry F      S aug-cc-pVQZ          selected for orbital group  1
 Library entry F      P aug-cc-pVQZ          selected for orbital group  1
 Library entry F      D aug-cc-pVQZ          selected for orbital group  1
 Library entry F      F aug-cc-pVQZ          selected for orbital group  1
 Library entry F      G aug-cc-pVQZ          selected for orbital group  1
 Library entry H      S aug-cc-pVQZ          selected for orbital group  2
 Library entry H      P aug-cc-pVQZ          selected for orbital group  2
 Library entry H      D aug-cc-pVQZ          selected for orbital group  2
 Library entry H      F aug-cc-pVQZ          selected for orbital group  2

1PROGRAM * SEWARD (Integral evaluation for generally contracted gaussian basis sets)     Author: Roland Lindh, 1990

 Geometry written to block  1 of record 700

 Orientation using atomic charges 
 Molecule type: Asymmetric top,     Order of principal axis = 2
 User-specified symmetry elements: X,Y
 Symmetry elements: X,Y

 Point group  C2v 



 ATOMIC COORDINATES

 NR  ATOM    CHARGE       X              Y              Z

   1  F       9.00    0.000000000    0.000000000    3.435865693
   2  H       1.00    0.000000000    0.700521477  -15.461395621
   3  H       1.00    0.000000000   -0.700521477  -15.461395621

 Bond lengths in Bohr (Angstrom)

 2-3  1.401042954
     ( 0.741400000)

 NUCLEAR CHARGE:                   11
 NUMBER OF PRIMITIVE AOS:         232
 NUMBER OF SYMMETRY AOS:          189
 NUMBER OF CONTRACTIONS:          172   (  61A1  +  35B1  +  49B2  +  27A2  )
 NUMBER OF CORE ORBITALS:           1   (   1A1  +   0B1  +   0B2  +   0A2  )
 NUMBER OF VALENCE ORBITALS:        6   (   3A1  +   1B1  +   2B2  +   0A2  )


 NUCLEAR REPULSION ENERGY    1.66561917


 Eigenvalues of metric

         1 0.528E-03 0.104E-02 0.173E-02 0.116E-01 0.127E-01 0.236E-01 0.294E-01 0.392E-01
         2 0.127E-01 0.294E-01 0.796E-01 0.101E+00 0.143E+00 0.193E+00 0.250E+00 0.250E+00
         3 0.314E-04 0.606E-04 0.458E-03 0.120E-02 0.574E-02 0.728E-02 0.108E-01 0.127E-01
         4 0.120E-02 0.728E-02 0.223E-01 0.286E-01 0.967E-01 0.143E+00 0.152E+00 0.243E+00


 Contracted 2-electron integrals neglected if value below      1.0D-12
 AO integral compression algorithm  1   Integral accuracy      1.0D-12

     47.972 MB (compressed) written to integral file ( 26.4%)

     Node minimum: 4.456 MB, node maximum: 8.913 MB


 NUMBER OF SORTED TWO-ELECTRON INTEGRALS:    3542697.     BUFFER LENGTH:  32768
 NUMBER OF SEGMENTS:   1  SEGMENT LENGTH:    3542697      RECORD LENGTH: 524288

 Memory used in sort:       4.10 MW

 SORT1 READ    22586686. AND WROTE      701180. INTEGRALS IN      3 RECORDS. CPU TIME:     0.35 SEC, REAL TIME:     0.40 SEC
 SORT2 READ     5623116. AND WROTE    28370651. INTEGRALS IN    160 RECORDS. CPU TIME:     0.10 SEC, REAL TIME:     0.13 SEC

 Node minimum:     3535778.  Node maximum:     3567689. integrals

 OPERATOR DM      FOR CENTER  0  COORDINATES:    0.000000    0.000000    0.000000


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        7.88       500      610      700      900      950      970     1000      129      960     1100   
                                          VAR    BASINP    GEOM    SYMINP    ZMAT    AOBASIS   BASIS     P2S    ABASIS      S 
                                         1400     1410     1200     1210     1080     1600     1650     1700   
                                           T        V       H0       H01     AOSYM     SMH    MOLCAS    OPER   

 PROGRAMS   *        TOTAL       INT
 CPU TIMES  *         1.55      1.13
 REAL TIME  *         2.82 SEC
 DISK USED  *       134.25 MB      
 GA USED    *         0.00 MB       (max)       0.00 MB       (current)
 **********************************************************************************************************************************

1PROGRAM * RHF-SCF (CLOSED SHELL)       Authors: W. Meyer, H.-J. Werner


 NUMBER OF ELECTRONS:       6+    6-    SPACE SYMMETRY=1    SPIN SYMMETRY: Singlet 
 CONVERGENCE THRESHOLDS:    1.00E-05 (Density)    1.00E-07 (Energy)
 MAX. NUMBER OF ITERATIONS:       60
 INTERPOLATION TYPE:            DIIS
 INTERPOLATION STEPS:              2 (START)      1 (STEP)
 LEVEL SHIFTS:                  0.00 (CLOSED)  0.00 (OPEN) 



 Orbital guess generated from atomic densities. Full valence occupancy:    4   1   2   0

 Molecular orbital dump at record        2140.2

 ITERATION    DDIFF          GRAD             ENERGY        2-EL.EN.            DIPOLE MOMENTS         DIIS   ORB.
    1      0.000D+00      0.000D+00      -100.49366820     98.088884    0.00000    0.00000   -3.43587    0    start
    2      0.000D+00      0.196D-01      -100.53006282     88.118183    0.00000    0.00000   -3.42645    1    diag
    3      0.160D-01      0.192D-01      -100.59075091     92.439451    0.00000    0.00000   -3.42525    2    diag
    4      0.728D-02      0.102D-02      -100.59090045     92.511842    0.00000    0.00000   -3.42356    3    diag
    5      0.440D-03      0.239D-03      -100.59091075     92.552988    0.00000    0.00000   -3.42312    4    diag
    6      0.109D-03      0.193D-04      -100.59091094     92.552314    0.00000    0.00000   -3.42300    5    diag
    7      0.208D-04      0.255D-05      -100.59091094     92.552682    0.00000    0.00000   -3.42299    6    diag
    8      0.180D-05      0.166D-06      -100.59091094     92.552704    0.00000    0.00000   -3.42299    0    orth

 Final occupancy:   4   1   1   0

 !RHF STATE 1.1 Energy               -100.590910944465
 Nuclear energy                         1.66561917
 One-electron energy                 -148.53288198
 Two-electron energy                   46.27635186
 Virial quotient                       -1.00014679
 !RHF STATE 1.1 Dipole moment           0.00000000     0.00000000    -3.42298614
 Dipole moment /Debye                   0.00000000     0.00000000    -8.69979311

 ELECTRON ORBITALS
 =================


   Orb  Occ    Energy  Couls-En    Coefficients

                                   1 1s      1 1s      1 1s      1 1s      1 1s      1 1s      1 2pz     1 2pz     1 2pz     1 2pz  
                                   1 2pz     1 3d0     1 3d2+    1 3d0     1 3d2+    1 3d0     1 3d2+    1 3d0     1 3d2+    1 4f0  
                                   1 4f2+    1 4f0     1 4f2+    1 4f0     1 4f2+    1 5g0     1 5g4+    1 5g2+    1 5g0     1 5g4+ 
                                   1 5g2+    2 1s      2 1s      2 1s      2 1s      2 1s      2 2pz     2 2py     2 2pz     2 2py  
                                   2 2pz     2 2py     2 2pz     2 2py     2 3d0     2 3d2+    2 3d1-    2 3d0     2 3d2+    2 3d1- 
                                   2 3d0     2 3d2+    2 3d1-    2 4f0     2 4f2+    2 4f1-    2 4f3-    2 4f0     2 4f2+    2 4f1- 
                                   2 4f3- 

   1.1   2   -25.8307  -66.3543  1.000258  0.000933 -0.000084 -0.000821  0.000255 -0.000251  0.000000 -0.000000 -0.000000 -0.000000
                                 0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000 -0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000  0.000000 -0.000000  0.000000
                                -0.000000  0.000000 -0.000000  0.000000 -0.000001  0.000000 -0.000000  0.000000  0.000000 -0.000000
                                -0.000000  0.000000  0.000000 -0.000001 -0.000000 -0.000000  0.000000 -0.000000 -0.000000 -0.000000
                                -0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000
                                 0.000000

   2.1   2    -1.0749   -9.9970 -0.001296  0.969626 -0.002311 -0.018283  0.039812  0.025748  0.000000  0.000000  0.000000  0.000000
                                 0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000  0.000000 -0.000000  0.000000
                                -0.000000 -0.000000  0.000001 -0.000001  0.000002 -0.000002 -0.000000 -0.000000  0.000000  0.000000
                                -0.000000 -0.000000  0.000000  0.000002  0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000
                                 0.000000  0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000

   3.1   2    -0.5416   -2.2703 -0.000000 -0.000000 -0.000000  0.000001 -0.000002  0.000002 -0.000000  0.000001 -0.000001  0.000004
                                -0.000005 -0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000
                                 0.000000  0.000000 -0.000000 -0.000000  0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000
                                -0.000000  1.153431 -0.030421 -0.205301 -0.206734 -0.000783 -0.000054 -0.007958 -0.000037 -0.016742
                                -0.001121 -0.014163 -0.001905 -0.006343 -0.001090 -0.001880  0.000006  0.000952  0.001633 -0.000008
                                 0.001013  0.002081  0.000105  0.000003  0.000003 -0.000126 -0.000165 -0.000017 -0.000008 -0.001024
                                -0.001319

   4.1   2    -0.1810   -7.8786 -0.000000 -0.000002 -0.000000  0.000001 -0.000002  0.000005  0.911992 -0.002200  0.003187  0.075043
                                 0.094483  0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000002  0.000000 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000  0.000000 -0.000000  0.000000 -0.000000
                                 0.000000 -0.000008  0.000047 -0.000074  0.000243 -0.000233  0.000000 -0.000006 -0.000001  0.000013
                                 0.000006 -0.000004 -0.000008  0.000203  0.000000  0.000001 -0.000000  0.000004  0.000006  0.000001
                                 0.000015  0.000027  0.000006 -0.000000 -0.000000 -0.000002 -0.000003  0.000002  0.000002 -0.000001
                                -0.000001

                                   1 2px     1 2px     1 2px     1 2px     1 2px     1 3d1+    1 3d1+    1 3d1+    1 3d1+    1 4f1+ 
                                   1 4f3+    1 4f1+    1 4f3+    1 4f1+    1 4f3+    1 5g1+    1 5g3+    1 5g1+    1 5g3+    2 2px  
                                   2 2px     2 2px     2 2px     2 3d1+    2 3d2-    2 3d1+    2 3d2-    2 3d1+    2 3d2-    2 4f1+ 
                                   2 4f3+    2 4f2-    2 4f1+    2 4f3+    2 4f2- 

   1.2   2    -0.1810   -7.8782  0.911992 -0.002200  0.003187  0.075043  0.094484  0.000000  0.000000 -0.000000  0.000001 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000  0.000000 -0.000000
                                 0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000 -0.000000  0.000000
                                 0.000000 -0.000000 -0.000000 -0.000000  0.000000

                                   1 2py     1 2py     1 2py     1 2py     1 2py     1 3d1-    1 3d1-    1 3d1-    1 3d1-    1 4f1- 
                                   1 4f3-    1 4f1-    1 4f3-    1 4f1-    1 4f3-    1 5g1-    1 5g3-    1 5g1-    1 5g3-    2 1s   
                                   2 1s      2 1s      2 1s      2 1s      2 2py     2 2pz     2 2py     2 2pz     2 2py     2 2pz  
                                   2 2py     2 2pz     2 3d1-    2 3d0     2 3d2+    2 3d1-    2 3d0     2 3d2+    2 3d1-    2 3d0  
                                   2 3d2+    2 4f1-    2 4f3-    2 4f0     2 4f2+    2 4f1-    2 4f3-    2 4f0     2 4f2+ 

   1.3   2    -0.1810   -7.8782  0.911991 -0.002200  0.003187  0.075043  0.094486  0.000000  0.000000 -0.000000  0.000001 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000002
                                -0.000006  0.000372  0.002638  0.000713 -0.000001 -0.000000  0.000013  0.000001 -0.000160  0.000013
                                -0.000613  0.000016 -0.000000  0.000001  0.000001 -0.000002 -0.000000 -0.000001 -0.000006 -0.000023
                                -0.000040 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000001 -0.000001

 HOMO      4.1    -0.180975 =      -4.9246eV
 LUMO      2.3     0.098334 =       2.6758eV
 LUMO-HOMO         0.279309 =       7.6004eV


 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      18        7.89       500      610      700      900      950      970     1000      129      960     1100   
                                          VAR    BASINP    GEOM    SYMINP    ZMAT    AOBASIS   BASIS     P2S    ABASIS      S 
                                         1400     1410     1200     1210     1080     1600     1650     1700   
                                           T        V       H0       H01     AOSYM     SMH    MOLCAS    OPER   

              2       4        0.51       700     1000      520     2140   
                                         GEOM     BASIS   MCVARS     RHF  

 PROGRAMS   *        TOTAL       RHF       INT
 CPU TIMES  *         1.69      0.15      1.13
 REAL TIME  *         3.18 SEC
 DISK USED  *       205.94 MB      
 SF USED    *         0.03 MB      
 GA USED    *         0.00 MB       (max)       0.00 MB       (current)
 **********************************************************************************************************************************

1PROGRAM * MULTI (Direct Multiconfiguration SCF)       Authors: P.J. Knowles, H.-J. Werner (1984)     S.T. Elbert (1988)


 Number of closed-shell orbitals:   1 (   1   0   0   0 )
 Number of active  orbitals:        6 (   3   1   2   0 )
 Number of external orbitals:     165 (  57  34  47  27 )

 State symmetry 1

 Number of electrons:    10    Spin symmetry=Singlet   Space symmetry=1
 Number of states:        1
 Number of CSFs:         10   (14 determinants, 36 intermediate states)

 Molecular orbitals read from record     2140.2  Type=RHF/CANONICAL (state 1.1)

 Wavefunction dump at record             2141.2

 Convergence thresholds  0.10E-01 (gradient)  0.10E-05 (energy)  0.10E-02 (step length)

 Number of orbital rotations:      359   (     3 Core/Active     57 Core/Virtual   0 Active/Active    299 Active/Virtual)
 Total number of variables:        373


 ITER. MIC  NCI  NEG     ENERGY(VAR)     ENERGY(PROJ)   ENERGY CHANGE     GRAD(0)  GRAD(ORB)   GRAD(CI)     STEP       TIME

   1   40    7    0    -100.59091558    -100.61196875   -0.02105318    0.00006704 0.00010284 0.00000000  0.92D+00      0.17
   2   33    5    0    -100.60884916    -100.60944674   -0.00059758    0.02838230 0.00000004 0.00000000  0.11D+00      0.29
   3   30    4    0    -100.60944672    -100.60944672   -0.00000000    0.00005097 0.00000005 0.00000000  0.18D-03      0.39

 ** WVFN ****  CONVERGENCE REACHED, FINAL GRADIENT:  0.46D-07


 First order charge density matrix for state 1.1 saved on record  2141.2 (density set 1)

 Results for state 1.1
 =====================

 !MCSCF STATE 1.1 Energy             -100.609446720328
 Nuclear energy                         1.66561917
 Kinetic energy                       100.61514722
 One electron energy                 -148.51853066
 Two electron energy                   46.24346477
 Virial ratio                           1.99994334

 !MCSCF STATE 1.1 Dipole moment         0.00000000     0.00000000    -3.42362136
 Dipole moment /Debye                   0.00000000     0.00000000    -8.70140759


 NATURAL ORBITALS
 ================

   Orb     Occ        Energy       Coefficients

                                   1 1s      1 1s      1 1s      1 1s      1 1s      1 1s      1 2pz     1 2pz     1 2pz     1 2pz  
                                   1 2pz     1 3d0     1 3d2+    1 3d0     1 3d2+    1 3d0     1 3d2+    1 3d0     1 3d2+    1 4f0  
                                   1 4f2+    1 4f0     1 4f2+    1 4f0     1 4f2+    1 5g0     1 5g4+    1 5g2+    1 5g0     1 5g4+ 
                                   1 5g2+    2 1s      2 1s      2 1s      2 1s      2 1s      2 2pz     2 2py     2 2pz     2 2py  
                                   2 2pz     2 2py     2 2pz     2 2py     2 3d0     2 3d2+    2 3d1-    2 3d0     2 3d2+    2 3d1- 
                                   2 3d0     2 3d2+    2 3d1-    2 4f0     2 4f2+    2 4f1-    2 4f3-    2 4f0     2 4f2+    2 4f1- 
                                   2 4f3- 

   1.1  2.00000   -25.830667     1.000258  0.000933 -0.000084 -0.000821  0.000255 -0.000251  0.000000 -0.000000 -0.000000 -0.000000
                                 0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000 -0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000  0.000000 -0.000000  0.000000
                                -0.000000  0.000000 -0.000000  0.000000 -0.000001  0.000000 -0.000000  0.000000  0.000000 -0.000000
                                -0.000000  0.000000  0.000000 -0.000001 -0.000000 -0.000000  0.000000 -0.000000 -0.000000 -0.000000
                                -0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000
                                 0.000000

   2.1  2.00000    -0.180979    -0.000000 -0.000001 -0.000000  0.000000 -0.000001  0.000003  0.911992 -0.002200  0.003187  0.075043
                                 0.094483  0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000001  0.000000 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000  0.000000 -0.000000  0.000000 -0.000000
                                 0.000000 -0.000017  0.000048 -0.000072  0.000244 -0.000233  0.000000 -0.000006 -0.000001  0.000013
                                 0.000006 -0.000003 -0.000008  0.000204  0.000000  0.000001 -0.000000  0.000004  0.000006  0.000001
                                 0.000015  0.000027  0.000006 -0.000000 -0.000000 -0.000002 -0.000003  0.000002  0.000002 -0.000001
                                -0.000001

   3.1  2.00000    -1.074939    -0.001296  0.969626 -0.002311 -0.018283  0.039812  0.025748  0.000000  0.000000  0.000000  0.000000
                                 0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000  0.000000
                                -0.000000 -0.000000  0.000001 -0.000001  0.000002 -0.000002 -0.000000 -0.000000  0.000000  0.000000
                                -0.000000 -0.000000  0.000000  0.000002  0.000000  0.000000  0.000000  0.000000  0.000000 -0.000000
                                 0.000000  0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000
                                 0.000000

   4.1  1.97590    -0.533737    -0.000000 -0.000000 -0.000000  0.000002 -0.000003  0.000003  0.000006  0.000001 -0.000002  0.000006
                                -0.000007 -0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000  0.000000 -0.000000 -0.000000
                                 0.000000  0.000000 -0.000000 -0.000000  0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000000
                                -0.000000  1.172213 -0.027913 -0.212634 -0.219653 -0.001124 -0.000057 -0.007318 -0.000051 -0.013606
                                -0.001159 -0.009499 -0.001776 -0.005012 -0.001031 -0.001778  0.000005  0.000802  0.001377 -0.000021
                                 0.000699  0.001523  0.000062  0.000003  0.000002  0.000009  0.000010 -0.000019 -0.000012 -0.000855
                                -0.001100

                                   1 2px     1 2px     1 2px     1 2px     1 2px     1 3d1+    1 3d1+    1 3d1+    1 3d1+    1 4f1+ 
                                   1 4f3+    1 4f1+    1 4f3+    1 4f1+    1 4f3+    1 5g1+    1 5g3+    1 5g1+    1 5g3+    2 2px  
                                   2 2px     2 2px     2 2px     2 3d1+    2 3d2-    2 3d1+    2 3d2-    2 3d1+    2 3d2-    2 4f1+ 
                                   2 4f3+    2 4f2-    2 4f1+    2 4f3+    2 4f2- 

   1.2  2.00000    -0.180979     0.911991 -0.002200  0.003187  0.075043  0.094485  0.000000  0.000000 -0.000000  0.000001 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000  0.000000 -0.000000
                                 0.000000 -0.000000  0.000000  0.000000  0.000000 -0.000000 -0.000000  0.000000 -0.000000  0.000000
                                 0.000000 -0.000000 -0.000000 -0.000000  0.000000

                                   1 2py     1 2py     1 2py     1 2py     1 2py     1 3d1-    1 3d1-    1 3d1-    1 3d1-    1 4f1- 
                                   1 4f3-    1 4f1-    1 4f3-    1 4f1-    1 4f3-    1 5g1-    1 5g3-    1 5g1-    1 5g3-    2 1s   
                                   2 1s      2 1s      2 1s      2 1s      2 2py     2 2pz     2 2py     2 2pz     2 2py     2 2pz  
                                   2 2py     2 2pz     2 3d1-    2 3d0     2 3d2+    2 3d1-    2 3d0     2 3d2+    2 3d1-    2 3d0  
                                   2 3d2+    2 4f1-    2 4f3-    2 4f0     2 4f2+    2 4f1-    2 4f3-    2 4f0     2 4f2+ 

   1.3  2.00000    -0.180979     0.911991 -0.002200  0.003187  0.075043  0.094486  0.000000  0.000000 -0.000000  0.000001 -0.000000
                                -0.000000  0.000000  0.000000 -0.000000 -0.000000 -0.000000 -0.000000  0.000000  0.000000  0.000002
                                -0.000006  0.000372  0.002638  0.000713 -0.000001 -0.000000  0.000013  0.000001 -0.000160  0.000013
                                -0.000613  0.000016 -0.000000  0.000001  0.000001 -0.000002 -0.000000 -0.000001 -0.000006 -0.000023
                                -0.000040 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000000 -0.000001 -0.000001

   2.3  0.02410     0.675159     0.000000 -0.000001  0.000003 -0.000008  0.000010  0.000000 -0.000000  0.000001 -0.000001  0.000000
                                -0.000000 -0.000000  0.000000  0.000000 -0.000000  0.000000 -0.000000 -0.000000  0.000000  1.870917
                                 0.298782  0.101666 -1.282165 -0.034146  0.005083 -0.000108 -0.034958 -0.000953 -0.054306 -0.002829
                                 0.160598 -0.000995  0.000007  0.000708  0.001229 -0.000147 -0.002442 -0.004160 -0.000402  0.002189
                                 0.004082 -0.000933 -0.001208 -0.000019 -0.000024 -0.000147 -0.000157 -0.000085 -0.000096

 Total charge:  -1.000000000000
 

 Natural orbital dump at molpro section  2141.2    (Orbital set 2)


 CI vector
 =========

 222 2 20       0.9939576
 220 2 22      -0.1097644

 TOTAL ENERGIES                      -100.60944672



 **********************************************************************************************************************************
 DATASETS  * FILE   NREC   LENGTH (MB)   RECORD NAMES
              1      19       10.64       500      610      700      900      950      970     1000      129      960     1100   
                                          VAR    BASINP    GEOM    SYMINP    ZMAT    AOBASIS   BASIS     P2S    ABASIS      S 
                                         1400     1410     1200     1210     1080     1600     1650     1700     1380   
                                           T        V       H0       H01     AOSYM     SMH    MOLCAS    OPER     JKOP   

              2       5        0.88       700     1000      520     2140     2141   
                                         GEOM     BASIS   MCVARS     RHF     MCSCF   

 PROGRAMS   *        TOTAL    CASSCF       RHF       INT
 CPU TIMES  *         2.19      0.49      0.15      1.13
 REAL TIME  *         4.01 SEC
 DISK USED  *       205.94 MB      
 SF USED    *        14.52 MB      
 GA USED    *         0.00 MB       (max)       0.00 MB       (current)
 **********************************************************************************************************************************

        CASSCF          RHF-SCF 
   -100.60944672   -100.59091094
 **********************************************************************************************************************************
 Variable memory released


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